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Design and development of extractants for radionuclides based on boron cluster anions

Project goals

The aim of the Project is continuation in the design and development of new extractants based on the derivatives of hydrophobic cluster boron ions for separation of fission products from nuclear waste, mainly actinides/ lanthanides (An/ Ln, eventually Csand Sr). The research will be directed to optimization of the molecular structures to enable good efficiency, easier stripping, solubility in less polar solvent systems, high chemical and radiation stability and selectivity, this for An will be particularly adressed. Another aim is deeper elucidation of the extraction mechanism using these ionic extractans and reflection of this knowledge into molecular design, especially in respect to easier re-extraction. Expected result is definition of several potentially interesting extractants, which would meet requirements for their direct application in the highly active nuclear waste technology and reprocessing of spent fuel from nuclear power stations. New sensors and analytical devices with high affinitiesand selectivities towards Ln and An can form additional output of the Project. A close interdisciplinary collaboration of Groups from the field of inorganic cluster synthesis with radiochemists specialized in separation methods, extraction studies and nuclear technology seems essential to fulfil the requirements of the Project.

Keywords

jaderné odpadyextrakce kapalina-kapalinakarboranymetallaborany

Public support

  • Provider

    Czech Science Foundation

  • Programme

    Standard projects

  • Call for proposals

    Standardní projekty 12 (SGA02009GA-ST)

  • Main participants

  • Contest type

    VS - Public tender

  • Contract ID

    104/09/0668

Alternative language

  • Project name in Czech

    Vývoj a optimalizace extrakčních činidel pro radionuklidy založených na borových klastrových aniontech

  • Annotation in Czech

    Projekt má za cíl pokračovat ve vývoj typů extračních činidel na bázi derivátů borových klastrových aniontů na základě originálních syntetických postupů. Činidla jsou navržena pro extrakci štěpných produktů, hlavně aktinidů/ lantahanidů (An/ Ln,popřípaděCs, Sr)z jaderných odpadů.

Scientific branches

  • R&D category

    ZV - Basic research

  • CEP classification - main branch

    DL - Nuclear waste, radioactive pollution and control

  • CEP - secondary branch

    CA - Inorganic chemistry

  • CEP - another secondary branch

    CB - Analytical chemistry, separation

  • 10402 - Inorganic and nuclear chemistry
    10406 - Analytical chemistry
    10511 - Environmental sciences (social aspects to be 5.7)

Completed project evaluation

  • Provider evaluation

    U - Uspěl podle zadání (s publikovanými či patentovanými výsledky atd.)

  • Project results evaluation

    The project gone according to plan both in terms of expertise and in terms of disbursement of funds.

Solution timeline

  • Realization period - beginning

    Jan 1, 2009

  • Realization period - end

    Dec 31, 2011

  • Project status

    U - Finished project

  • Latest support payment

    Apr 16, 2011

Data delivery to CEP

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

  • Data delivery code

    CEP12-GA0-GA-U/02:2

  • Data delivery date

    May 2, 2016

Finance

  • Total approved costs

    5,651 thou. CZK

  • Public financial support

    3,779 thou. CZK

  • Other public sources

    0 thou. CZK

  • Non public and foreign sources

    1,872 thou. CZK