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Ring-substituted polyphenylacetylenes prepared with insertion catalysts: preparation, characterization, study of molecular weight and configurational stability

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F10%3A10062572" target="_blank" >RIV/00216208:11310/10:10062572 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Ring-substituted polyphenylacetylenes prepared with insertion catalysts: preparation, characterization, study of molecular weight and configurational stability

  • Original language description

    Series of fluorine-containing ring-substituted phenylacetylenes have been polymerized with various Rh based catalysts. In polymerization systems yielding the soluble products we achieved the MW control by a proper selection of Rh-catalyst composition. All the prepared soluble polymers were of high microstructure uniformity with high cis double bonds content. Selected samples were submitted to the long-term MW and configurational stability tests. Polymers dissolved in THF and exposed to the atmosphere atdiffused day light had undergone simultaneously proceeding cis-to-trans isomerisation and degradation. The stability of polymers was positively affected by the bulkiness of substituent on the Ph-ring and by the presence of substituent in the vicinity ofthe polymer main chain. The detailed study of ageing process involving the analyses of deeply aged polymer samples revealed the non-random character of degradation and mutual interconnection of degradation and cis-to-trans isomerisation

  • Czech name

  • Czech description

Classification

  • Type

    D - Article in proceedings

  • CEP classification

    CD - Macromolecular chemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>Z - Vyzkumny zamer (s odkazem do CEZ)<br>S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2010

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    10th Pannonian Symposium on Catalysis

  • ISBN

    978-83-929430-4-4

  • ISSN

  • e-ISSN

  • Number of pages

    8

  • Pages from-to

  • Publisher name

    Polish Zeolite Association and Institute of Catalysis and Surface Chemistry

  • Place of publication

    Kraków, Poland

  • Event location

    Kraków, Poland

  • Event date

    Aug 29, 2010

  • Type of event by nationality

    EUR - Evropská akce

  • UT code for WoS article