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Chain-Growth Insertion Polymerization of 1,3-Diethynylbenzene High Internal Phase Emulsions into Reactive ? - Conjugated Foams

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F14%3A10271602" target="_blank" >RIV/00216208:11310/14:10271602 - isvavai.cz</a>

  • Result on the web

    <a href="http://pubs.acs.org/doi/pdf/10.1021/ma501142d" target="_blank" >http://pubs.acs.org/doi/pdf/10.1021/ma501142d</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/ma501142d" target="_blank" >10.1021/ma501142d</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Chain-Growth Insertion Polymerization of 1,3-Diethynylbenzene High Internal Phase Emulsions into Reactive ? - Conjugated Foams

  • Original language description

    The ?-conjugated micro/macroporous polyacetylene-type polyHIPE foams were synthesized for the fi rst time by a chain-growth insertion polymerization of high internal phase emulsions (HIPEs). In the first step, the ?-conjugated polyHIPE foams were prepared by polymerization of 1,3-diethynylbenzene HIPEs using [Rh(nbd)acac] complex as a catalyst. The ? -conjugated polyHIPE foams consist of ethynylphenyl-substituted polyene main chains which are cross-linked by the 1,3-phenylene linkers. In the second step, the foams were chemically and thermally postmodified by applying the alkyneMINUS SIGN azide cycloaddition reaction and the solvent free solid phase hyper-cross-linking at temperature of 280oC. Thus, obtained polyacetylene-type polyHIPE foams exhibit hierarchically structured micro/macroporous morphology with sizes of the macropores and interconnecting pores of 3.4 +- 0.3 ?m (or 4.8 +- 0.8 ?m) and 0.96 ?m (or 1.1 ?m), respectively, wherein a substantial volume of micropores is also foun

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CD - Macromolecular chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GAP108%2F11%2F1661" target="_blank" >GAP108/11/1661: Organic nanoporous polymers derived from arylacetylenes as materials for hydrogen storage</a><br>

  • Continuities

    S - Specificky vyzkum na vysokych skolach<br>I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Macromolecules

  • ISSN

    0024-9297

  • e-ISSN

  • Volume of the periodical

    47

  • Issue of the periodical within the volume

    15

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    6

  • Pages from-to

    4864-4869

  • UT code for WoS article

    000340350400003

  • EID of the result in the Scopus database