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Geochemical sources, forms and phases of soil contamination in an industrial city

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F17%3A10360017" target="_blank" >RIV/00216208:11310/17:10360017 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.scitotenv.2017.01.053" target="_blank" >http://dx.doi.org/10.1016/j.scitotenv.2017.01.053</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.scitotenv.2017.01.053" target="_blank" >10.1016/j.scitotenv.2017.01.053</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Geochemical sources, forms and phases of soil contamination in an industrial city

  • Original language description

    This study examines current soil contamination in an Australian industrial city, Newcastle. Public (roadside verges and parks) and private (homes) surface soils (n = 170) contained metal(loid)s elevated above their respective Australian Health Investigation Levels (HIL). Lead (Pb), the most common contaminant in the city, exceeds the HIL for residential soils (HIL-A, 300 mg/kg) in 88% of private soils (median: 1140 mg/kg). In-vitro Pb bio-accessibility analysis of selected soils (n = 11) using simulated gastric fluid showed a high affinity for Pb solubilisation (maximum Pb concentration: 5190 mg/kg, equating to 45% Pb bio-accessibility). Highly soluble Pb-laden Fe- and Mn-oxides likely contribute to the bio-accessibility of the Pb. Public and private space surface soils contain substantially less radiogenic Pb (range: Pb-208/Pb-207: 2.345-2.411, Pb-206/Pb-207: 1.068-1.312) than local background soil (Pb-208/Pb-207: 2.489, Pb-206/Pb-207: 1.198), indicating anthropogenic contamination from the less radiogenic Broken Hill type Pb ores (Pb-208/Pb-207: 2.319, Pb-206/Pb-207: 1.044). Source apportionment using Pb isotopic ratio quantification and soil mineralogy indicate the city&apos;s historic copper and steel industries contributed the majority of the soil contaminants through atmospheric deposition and use of slag waste as fill material. High-temperature silicates and oxides combined with rounded particles in the soil are characteristic of smelter dust emissions. Additionally, a preliminary investigation of polycyclic aromatic hydrocarbons in soils, sometimes associated with ferrous metal smelting, coal processing or burning Of fossil fuels, shows that these too pose a health exposure risk (calculated in comparison to benzo(a)pyrene: n = 12, max: 13.5 mg/kg, HIL: 3 mg/kg).

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10505 - Geology

Result continuities

  • Project

    <a href="/en/project/GA13-17501S" target="_blank" >GA13-17501S: Reactivity of anthropogenic metal-bearing geomaterials in soils</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Science of the Total Environment

  • ISSN

    0048-9697

  • e-ISSN

  • Volume of the periodical

    584

  • Issue of the periodical within the volume

    APRIL

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    10

  • Pages from-to

    505-514

  • UT code for WoS article

    000399358500049

  • EID of the result in the Scopus database

    2-s2.0-85014864609