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Voltammetric and adsorption study of 4-nitrophenyl-triazole-labeled 2'-deoxycytidine and 7-deazaadenosine nucleosides at boron-doped diamond electrode

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F18%3A10378037" target="_blank" >RIV/00216208:11310/18:10378037 - isvavai.cz</a>

  • Alternative codes found

    RIV/68081707:_____/18:00500229 RIV/61388963:_____/18:00500229 RIV/00216224:14740/18:00101395

  • Result on the web

    <a href="https://doi.org/10.1016/j.jelechem.2018.01.003" target="_blank" >https://doi.org/10.1016/j.jelechem.2018.01.003</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.jelechem.2018.01.003" target="_blank" >10.1016/j.jelechem.2018.01.003</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Voltammetric and adsorption study of 4-nitrophenyl-triazole-labeled 2'-deoxycytidine and 7-deazaadenosine nucleosides at boron-doped diamond electrode

  • Original language description

    Electrochemical properties of 4-nitrophenyl triazole labeled 2&apos;-deoxycytidine (dCTRN 2) and 7-deazaadenosine (dA(TRNO2)) were studied using alumina-polished boron doped diamond (BDD) electrode in acetate buffer pH 5.0. Cyclic voltammetry revealed peak-shaped signals for reduction of the nitro group at the potentials of ca -0.6 V (vs. AllAgCl13 mol L-1 KCl reference electrode) and for the hydroxylamine/nitroso pair exhibiting quasireversible electron transfer at potentials comparable with redox processes of other nitro aromatic compounds at BDD electrodes. All electrochemical processes are directed by adsorption. Moreover, ex situ adsorption of dA(TRNO2) and transfer to supporting electrolyte enables its quantitation using square wave voltammetry in small (several microliter) sample volumes after optimization of parameters for the hydroxylamine/nitroso redox couple. Competitive adsorption/desorption at the BDD surface was further studied by cyclic voltammetry with dA(TRNO2) in the presence of electrochemically inactive phenyl triazole 7-deazaadenosine conjugate (dA(TR)), revealing mutual displacement of both compounds at BDD surface. Further, the redox processes of simpler aromatic nitro compounds (4-nitrophenyl acetylene and 2-nitronaphthalene) are strongly affected when the BDD surface is covered by dA(TR).

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10406 - Analytical chemistry

Result continuities

  • Project

    <a href="/en/project/GBP206%2F12%2FG151" target="_blank" >GBP206/12/G151: Center of novel approaches to bioanalysis and molecular diagnostics</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2018

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Electroanalytical Chemistry

  • ISSN

    1572-6657

  • e-ISSN

  • Volume of the periodical

    821

  • Issue of the periodical within the volume

    July

  • Country of publishing house

    CH - SWITZERLAND

  • Number of pages

    10

  • Pages from-to

    111-120

  • UT code for WoS article

    000437818600018

  • EID of the result in the Scopus database

    2-s2.0-85042624643