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Ultrafast Light-Induced Ferromagnetic State in Transition Metal Dichalcogenides Monolayers

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F22%3A10450567" target="_blank" >RIV/00216208:11310/22:10450567 - isvavai.cz</a>

  • Result on the web

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=2gknF5Fn5T" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=2gknF5Fn5T</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.jpclett.2c00443" target="_blank" >10.1021/acs.jpclett.2c00443</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Ultrafast Light-Induced Ferromagnetic State in Transition Metal Dichalcogenides Monolayers

  • Original language description

    Ultrafast optical control of magnetism had great potential to revolutionizemagnetic storage technology and spintronics, but for now, its potential remains mostlyuntapped in two-dimensional (2D) magnets. Here, using the state-of-the-art real-time time-dependent density functional theory (rt-TDDFT), we demonstrate that an ultrafast laser pulsecan induce a ferromagnetic state in nonmagnetic MoSe2monolayers interfaced with van derWaals (vdW) ferromagnetic MnSe2. Our results show that the transient ferromagnetism inMoSe2derives from photoinduced direct ultrafast interlayer spin transfer from Mn to Mo via avdW-coupled interface, albeit with a delay of approximately a few femtoseconds. This delaywas strongly dependent on laser duration and interlayer coupling, which could be used to tunethe amplitude and rate spin transfer. Furthermore, we have also shown that ferromagneticstates can be photoinduced in other transition metal dichalcogenides (TMDs), such as PtS2and TaSe2monolayers. Overall, ourfindings provide crucial physical insights for exploringlight-induced interlayer spin and charge dynamics in 2D magnetic systems

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2022

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Physical Chemistry Letters

  • ISSN

    1948-7185

  • e-ISSN

    1948-7185

  • Volume of the periodical

    13

  • Issue of the periodical within the volume

    12

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    7

  • Pages from-to

    2765-2771

  • UT code for WoS article

    000783184700015

  • EID of the result in the Scopus database

    2-s2.0-85127567340