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Synthesis of Cationic [4], [5], and [6]Azahelicenes with Extended pi-Conjugated Systems

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F23%3A10465374" target="_blank" >RIV/00216208:11310/23:10465374 - isvavai.cz</a>

  • Result on the web

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=~_xrD.0UF4" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=~_xrD.0UF4</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.3390/catal13050912" target="_blank" >10.3390/catal13050912</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Synthesis of Cationic [4], [5], and [6]Azahelicenes with Extended pi-Conjugated Systems

  • Original language description

    The scope of Rh-catalyzed C-C bond cleavage/annulation of biphenylene with various aromatic nitriles was studied. The subsequent Rh- and Ir-catalyzed C-H bond activation/annulation sequence of the formed 9-arylphenanthridines with alkynes gave rise to cationic [4], [5], [6] helical quinolizinium salts. The scope of the reaction with respect to the structural features of the starting 9-arylphenanthridines and alkynes was studied. Their helical arrangement was confirmed through single-crystal X-ray analyses of selected compounds. Most of the prepared quinolizinium salts exhibited fluorescence emission maxima in the region of 525-623 nm with absolute quantum yields up to 25%.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10401 - Organic chemistry

Result continuities

  • Project

    <a href="/en/project/GA21-29124S" target="_blank" >GA21-29124S: REAP and Other Catalytic Reactions in Synthesis of Nitrogen-Embbeded Polyaromatic Hydrocarbons</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Catalysts

  • ISSN

    2073-4344

  • e-ISSN

    2073-4344

  • Volume of the periodical

    13

  • Issue of the periodical within the volume

    5

  • Country of publishing house

    CH - SWITZERLAND

  • Number of pages

    12

  • Pages from-to

    912

  • UT code for WoS article

    000997902000001

  • EID of the result in the Scopus database

    2-s2.0-85160728391