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Cross-tunneling and phonon bottleneck effects in the relaxation phenomena of XY pyrochlore antiferromagnet Er2Ti2O7

Result description

A multiple time scale relaxation dynamic is revealed by alternating current (ac) susceptibility studies of a single crystal of Er2Ti2O7 performed at high temperatures (k(B)T >> J/k(B)) in a wide range of static magnetic fields. An analysis of the frequency dependence of the ac susceptibility revealed the existence of two relaxationmechanisms, identified as an Orbach process with the pronounced effect of a phonon bottleneck and cross-tunneling. The origin of the phonon bottleneck is attributed to resonant phonon trapping. The relevance of the obtained results for relaxation phenomena found in other rare-earth pyrochlores, studied under similar conditions, is discussed.

Keywords

statesystemsdiffusionicedynamicscrystal-structurespin-lattice-relaxation

The result's identifiers

Alternative languages

  • Result language

    angličtina

  • Original language name

    Cross-tunneling and phonon bottleneck effects in the relaxation phenomena of XY pyrochlore antiferromagnet Er2Ti2O7

  • Original language description

    A multiple time scale relaxation dynamic is revealed by alternating current (ac) susceptibility studies of a single crystal of Er2Ti2O7 performed at high temperatures (k(B)T >> J/k(B)) in a wide range of static magnetic fields. An analysis of the frequency dependence of the ac susceptibility revealed the existence of two relaxationmechanisms, identified as an Orbach process with the pronounced effect of a phonon bottleneck and cross-tunneling. The origin of the phonon bottleneck is attributed to resonant phonon trapping. The relevance of the obtained results for relaxation phenomena found in other rare-earth pyrochlores, studied under similar conditions, is discussed.

  • Czech name

  • Czech description

Classification

  • Type

    Jx - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    BM - Solid-state physics and magnetism

  • OECD FORD branch

Result continuities

Others

  • Publication year

    2016

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    PHYSICAL REVIEW B

  • ISSN

    2469-9950

  • e-ISSN

  • Volume of the periodical

    93

  • Issue of the periodical within the volume

    2

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    9

  • Pages from-to

  • UT code for WoS article

    000368294500006

  • EID of the result in the Scopus database

    2-s2.0-84955263013

Basic information

Result type

Jx - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

Jx

CEP

BM - Solid-state physics and magnetism

Year of implementation

2016