Ultrafast Molecular Three-Electron Auger Decay
The result's identifiers
Result code in IS VaVaI
<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F16%3A10335810" target="_blank" >RIV/00216208:11320/16:10335810 - isvavai.cz</a>
Result on the web
<a href="http://dx.doi.org/10.1103/PhysRevLett.116.073001" target="_blank" >http://dx.doi.org/10.1103/PhysRevLett.116.073001</a>
DOI - Digital Object Identifier
<a href="http://dx.doi.org/10.1103/PhysRevLett.116.073001" target="_blank" >10.1103/PhysRevLett.116.073001</a>
Alternative languages
Result language
angličtina
Original language name
Ultrafast Molecular Three-Electron Auger Decay
Original language description
Three-electron Auger decay is an exotic and elusive process, in which two outer-shell electrons simultaneously refill an inner-shell double vacancy with emission of a single Auger electron. Such transitions are forbidden by the many-electron selection rules, normally making their decay lifetimes orders of magnitude longer than the few-femtosecond lifetimes of normal (two-electron) Auger decay. Here we present theoretical predictions and direct experimental evidence for a few-femtosecond three-electron Auger decay of a double inner-valence-hole state in CH3F. Our analysis shows that in contrast to double core holes, double inner-valence vacancies in molecules can decay exclusively by this ultrafast three-electron Auger process, and we predict that this phenomenon occurs widely.
Czech name
—
Czech description
—
Classification
Type
J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)
CEP classification
BG - Nuclear, atomic and molecular physics, accelerators
OECD FORD branch
—
Result continuities
Project
<a href="/en/project/GAP208%2F12%2F0521" target="_blank" >GAP208/12/0521: Non-radiative relaxation processes in ionized atomic and molecular systems</a><br>
Continuities
P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)
Others
Publication year
2016
Confidentiality
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů
Data specific for result type
Name of the periodical
Physical Review Letters
ISSN
0031-9007
e-ISSN
—
Volume of the periodical
116
Issue of the periodical within the volume
7
Country of publishing house
US - UNITED STATES
Number of pages
5
Pages from-to
—
UT code for WoS article
000370622000004
EID of the result in the Scopus database
2-s2.0-84959421898