Experimental quantification of site-specific efficiency of Interatomic Coulombic Decay after inner shell ionization
The result's identifiers
Result code in IS VaVaI
<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F23%3A10477093" target="_blank" >RIV/00216208:11320/23:10477093 - isvavai.cz</a>
Result on the web
<a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=h1oUfuhIe9" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=h1oUfuhIe9</a>
DOI - Digital Object Identifier
<a href="http://dx.doi.org/10.1038/s42005-023-01166-4" target="_blank" >10.1038/s42005-023-01166-4</a>
Alternative languages
Result language
angličtina
Original language name
Experimental quantification of site-specific efficiency of Interatomic Coulombic Decay after inner shell ionization
Original language description
Energy and charge transfer processes like Interatomic Coulombic Decay (ICD) play an important role in the relaxation of excited atoms or molecules in dense media such as biological tissue. Here, we present a method to experimentally determine the site-specific efficiency of the ICD process, which is in quantitative agreement with theoretical calculations. Interatomic Coulombic Decay (ICD) and related interatomic and intermolecular autoionization mechanisms are ubiquitous decay processes of excited atoms and molecules in an environment. It is commonly accepted that the efficiency of ICD of an ionized atom in a cluster increases with an increasing number of nearest neighbors. Here, we present a method for experimental validation of this assumption by a site-specific and quantitative comparison of ICD and its main competitor, Auger decay, in core-level ionized Kr clusters. Our results are in quantitative agreement with scaled theoretical calculations on Kr-2.
Czech name
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Czech description
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Classification
Type
J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database
CEP classification
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OECD FORD branch
10300 - Physical sciences
Result continuities
Project
<a href="/en/project/GA22-22658S" target="_blank" >GA22-22658S: Multi-electron decay processes in polyatomic systems</a><br>
Continuities
P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)
Others
Publication year
2023
Confidentiality
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů
Data specific for result type
Name of the periodical
Communications Physics
ISSN
2399-3650
e-ISSN
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Volume of the periodical
6
Issue of the periodical within the volume
1
Country of publishing house
GB - UNITED KINGDOM
Number of pages
5
Pages from-to
50
UT code for WoS article
000953886100001
EID of the result in the Scopus database
2-s2.0-85150411826