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Experimental and Theoretical Studies of Gas Phase Ion Mobility and Energetics: Protonated Saturated and Unsaturated Aldehydes in Helium

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F23%3A10478011" target="_blank" >RIV/00216208:11320/23:10478011 - isvavai.cz</a>

  • Result on the web

    <a href="https://physics.mff.cuni.cz/wds/proc/pdf23/WDS23_35_f2_OmezzineGnioua.pdf" target="_blank" >https://physics.mff.cuni.cz/wds/proc/pdf23/WDS23_35_f2_OmezzineGnioua.pdf</a>

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Experimental and Theoretical Studies of Gas Phase Ion Mobility and Energetics: Protonated Saturated and Unsaturated Aldehydes in Helium

  • Original language description

    Theoretical calculations and experimental measurements were carried out forselected classes of volatile organic compounds (VOC) to further understand the ion-molecule reactions important for mass spectrometric trace gas analysis. Quantumchemistry calculations based on the density functional theory, DFT, were performedusing the ORCA software to study the structures and energetics of protonated aldehydeions. The total enthalpies of the neutral and protonated molecules were calculated at theB3LYP 6-311++G(d,p) level of theory including the D4 dispersion correction for thestandard temperature and pressure. Proton affinities were thus obtained for pentanal,heptanal, octanal, 2-pentenal, 2-heptenal and 2-octenal. The Selected Ion Flow Drift TubeMass Spectrometry (SIFDT-MS) was used to measure the mobilities and energies ofprotonated aldehyde ions under different reduced electric field intensities (E/N) and theresults were compared with theoretical values based on the calculated ion geometries.

  • Czech name

  • Czech description

Classification

  • Type

    D - Article in proceedings

  • CEP classification

  • OECD FORD branch

    10305 - Fluids and plasma physics (including surface physics)

Result continuities

  • Project

  • Continuities

    S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    WDS&apos;23 Proceedings of Contributed Papers - Physics

  • ISBN

    978-80-7378-503-1

  • ISSN

  • e-ISSN

  • Number of pages

    7

  • Pages from-to

    244-250

  • Publisher name

    Matfyzpress

  • Place of publication

    Praha

  • Event location

    Praha

  • Event date

    May 30, 2023

  • Type of event by nationality

    EUR - Evropská akce

  • UT code for WoS article