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Pure TeO2 glass: Influence of synthesis conditions on linear and non-linear optical, magneto-optical and structural properties

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F24%3A10484471" target="_blank" >RIV/00216208:11320/24:10484471 - isvavai.cz</a>

  • Alternative codes found

    RIV/44555601:13440/24:43898419 RIV/44555601:13520/24:43898419 RIV/00216275:25310/24:39921921

  • Result on the web

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=Qo7J79l15I" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=Qo7J79l15I</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.jallcom.2024.174788" target="_blank" >10.1016/j.jallcom.2024.174788</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Pure TeO2 glass: Influence of synthesis conditions on linear and non-linear optical, magneto-optical and structural properties

  • Original language description

    The first systematic study of linear and non-linear optical, magneto-optical and structural properties of pure TeO(2) glass is presented with regard to different synthesis and material processing conditions. Prepared glasses were synthesized by the intermittent quenching from 900 °C in platinum or alumina crucibles and characterized prior to and after optical polishing. The position of the long-wavelength/phonon absorption edge was investigated using various optical models and experimentally obtained data of refractive index and Verdet constants were used for the estimation of magneto-optical anomaly parameter. During synthesis in alumina crucible, up to about 11 wt.% of Al(2)O(3) incorporates into the glass (verified by EDS/XRF and Raman/FTIR spectroscopy) partially transforming the original pure TeO(2) glass backbone structure composed of [TeO(4)] trigonal bipyramids to [TeO(3+1)] and [TeO(3)] structural units with the expected integration of Al into Te-O-Al bridges. The presence of Al(2)O(3) results in lowered density rho (5.60 -&gt; 4.72 g cm(-3)), refractive index n(1550) (2.086 -&gt; 1.927) and Verdet constant V(632) (36.3 -&gt; 21.9 rad T(-1) m(-1)) and in increased optical-band-gap energy E(g) (3.69 -&gt; 3.72 eV) and Abbe number nu(D) (19.9 -&gt; 26.9) compared to pure TeO(2) glass prepared in platinum crucible. A dataset of the obtained complex optical parameters (refractive index and extinction coefficient) in the wide spectral range of 193 11000 nm is included in the supplementary part.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10302 - Condensed matter physics (including formerly solid state physics, supercond.)

Result continuities

  • Project

    <a href="/en/project/LM2023066" target="_blank" >LM2023066: Nanomaterials and Nanotechnologies for Environment Protection and Sustainable Future</a><br>

  • Continuities

    S - Specificky vyzkum na vysokych skolach<br>I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Alloys and Compounds

  • ISSN

    0925-8388

  • e-ISSN

    1873-4669

  • Volume of the periodical

    997

  • Issue of the periodical within the volume

    30 August 2024

  • Country of publishing house

    CH - SWITZERLAND

  • Number of pages

    10

  • Pages from-to

    174788

  • UT code for WoS article

    001245529300001

  • EID of the result in the Scopus database

    2-s2.0-85193901389