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Shedding Light on the Origin of 204Pb, the Heaviest s-Process-Only Isotope in the Solar System

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F24%3A10494225" target="_blank" >RIV/00216208:11320/24:10494225 - isvavai.cz</a>

  • Result on the web

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=hj8vHGmpnn" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=hj8vHGmpnn</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1103/PhysRevLett.133.052702" target="_blank" >10.1103/PhysRevLett.133.052702</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Shedding Light on the Origin of 204Pb, the Heaviest s-Process-Only Isotope in the Solar System

  • Original language description

    Asymptotic giant branch stars are responsible for the production of most of the heavy isotopes beyond Srobserved in the solar system. Among them, isotopes shielded from the r-process contribution by their stableisobars are defined as s-only nuclei. For a long time the abundance of 204Pb, the heaviest s-only isotope, hasbeen a topic of debate because state-of-the-art stellar models appeared to systematically underestimate itssolar abundance. Besides the impact of uncertainties from stellar models and galactic chemical evolutionsimulations, this discrepancy was further obscured by rather divergent theoretical estimates for the neutroncapture cross section of its radioactive precursor in the neutron-capture flow, 204Tl (t1=21/4 3.78 yr), and bythe lack of experimental data on this reaction. We present the first ever neutron capture measurement on204Tl, conducted at the CERN neutron time-of-flight facility n_TOF, employing a sample of only 9 mg of204Tl produced at the Institute Laue Langevin high flux reactor. By complementing our new results withsemiempirical calculations we obtained, at the s-process temperatures of kT ALMOST EQUAL TO 8 keV and kT ALMOST EQUAL TO 30 keV,Maxwellian-averaged cross sections (MACS) of 580(168) mb and 260(90) mb, respectively. These figuresare about 3% lower and 20% higher than the corresponding values widely used in astrophysicalcalculations, which were based only on theoretical calculations. By using the new 204Tl MACS, theuncertainty arising from the 204Tlðn; γÞ cross section on the s-process abundance of 204Pb has been reducedfrom TILDE OPERATOR+D9130% down to þ8%= - 6%, and the s-process calculations are in agreement with the latest solarsystem abundance of 204Pb reported by K. Lodders in 2021.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10300 - Physical sciences

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Physical Review Letters

  • ISSN

    0031-9007

  • e-ISSN

    1079-7114

  • Volume of the periodical

    133

  • Issue of the periodical within the volume

    05

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    8

  • Pages from-to

    052702

  • UT code for WoS article

    001310903800008

  • EID of the result in the Scopus database

    2-s2.0-85201738849