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Elastic deformation suppresses ion demixing in mixed-halide perovskites

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F25%3A10504954" target="_blank" >RIV/00216208:11320/25:10504954 - isvavai.cz</a>

  • Alternative codes found

    RIV/68407700:21230/25:00389170 RIV/00216224:14310/25:00143351

  • Result on the web

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=t7ovRXYx9y" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=t7ovRXYx9y</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.matdes.2025.114850" target="_blank" >10.1016/j.matdes.2025.114850</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Elastic deformation suppresses ion demixing in mixed-halide perovskites

  • Original language description

    We simulated the kinetics of ion demixing in mixed-halide perovskites using phenomenological Cahn-Hilliard equation. In the model we considered the chemical and the elastic parts of Helmholtz free energy of the perovskite lattice, as well as the effect of free carriers generated by sample illumination. If the demixing process is accompanied by local elastic deformation caused by the dependence of the lattice parameter on the local chemical composition, the elastic contribution to the free energy is larger than the other two parts so that elastic deformation effectively suppresses the ion segregation. The demixing can take place if the internal stresses are relieved by surface elastic relaxation, or if the deformation of the lattice is plastic like around structural defects or at grain boundaries.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

    <a href="/en/project/GA23-06543S" target="_blank" >GA23-06543S: Structural changes induced by light soaking in mixed-halide perovskites</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2025

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Materials and Design

  • ISSN

    0264-1275

  • e-ISSN

    1873-4197

  • Volume of the periodical

    259

  • Issue of the periodical within the volume

    listopad

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    10

  • Pages from-to

    114850

  • UT code for WoS article

    001601382000011

  • EID of the result in the Scopus database

    2-s2.0-105020571468