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15N NMR study of N7- and N9-substituted purine derivatives

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216224%3A14310%2F02%3A00006185" target="_blank" >RIV/00216224:14310/02:00006185 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    15N NMR study of N7- and N9-substituted purine derivatives

  • Original language description

    Since 15N NMR parameters are sensitive indicators of the structural and electronic arrangements in organic compounds2 we used 15N NMR spectroscopy for investigating a set of N7- and N9-substituted purine analogues. The 15N NMR chemical shifts of N7- andN9-purine derivatives were investigated systematically at the natural abundance level of the 15N isotope. The NMR chemical shifts were determined and assigned using GSQMBC, GHMBC, GHMQC, and GHSQC experiments in solution. 15N CP/MAS data were recorded for selected compounds in order to study the principal values of the 15N chemical shifts. Geometric parameters obtained by using RHF/6-31G** and single-crystal X-ray structural analysis were used to calculate the chemical-shielding constants (GIAO and IGLO) which were then used to assign the nitrogen resonances observed in the solid-state NMR spectra and to determine the orientation of the principal components of the shift tensors.

  • Czech name

  • Czech description

Classification

  • Type

    D - Article in proceedings

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/LN00A016" target="_blank" >LN00A016: BIOMOLECULAR CENTER</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2002

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    16th European Experimental Nuclear Magnetic Resonance Conference

  • ISBN

    80-86186-07-5

  • ISSN

  • e-ISSN

  • Number of pages

    1

  • Pages from-to

    "PB129"

  • Publisher name

    Institute of Chemical Process Fundamentals, AS CR

  • Place of publication

    Prague

  • Event location

    June 9-14, Prague

  • Event date

  • Type of event by nationality

    WRD - Celosvětová akce

  • UT code for WoS article