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Two single-enantiomer amidophosphoesters: a database study on the chirality of (O)(2)P(O)(N)-based structures

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216224%3A14310%2F19%3A00109265" target="_blank" >RIV/00216224:14310/19:00109265 - isvavai.cz</a>

  • Result on the web

    <a href="http://scripts.iucr.org/cgi-bin/paper?S205322961801673X" target="_blank" >http://scripts.iucr.org/cgi-bin/paper?S205322961801673X</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1107/S205322961801673X" target="_blank" >10.1107/S205322961801673X</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Two single-enantiomer amidophosphoesters: a database study on the chirality of (O)(2)P(O)(N)-based structures

  • Original language description

    The crystal structures of two single-enantiomer amidophosphoesters with an (O)(2)P(O)(N) skeleton, i. e. diphenyl [(R)-(+)-alpha-methylbenzylamido] phosphate, (I), and diphenyl [(S)-(-)-alpha-methylbenzylamido] phosphate, (II), both C20H20-NO3P, are reported. In both structures, chiral one-dimensional hydrogenbonded architectures, along [010], are mediated by N-H center dot center dot center dot OP interactions. The statistically identical assemblies include the noncentrosymmetric graph-set motif C(4) and the compounds crystallize in the chiral space group P21. As a result of synergistic co-operation from C-H center dot center dot center dot O interactions, a two-dimensional superstructure is built including a noncentrosymmetric R-4(4)(22) hydrogenbonded motif. A Cambridge Structural Database survey was performed on (O)(2)P(O)(N)-based structures in order to review the frequency of space groups observed in this family of compounds; the hydrogen-bond motifs in structures with chiral space groups and the types of groups inducing chirality are discussed. The (2,3)J(X-P) (X = H or C) coupling constants from the NMR spectra of (I) and (II) have been studied. In each compound, the two diastereotopic C6H5O groups are different, which is reflected in the different chemical shifts and some coupling constants.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10400 - Chemical sciences

Result continuities

  • Project

  • Continuities

    S - Specificky vyzkum na vysokych skolach<br>I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    ACTA CRYSTALLOGRAPHICA SECTION C-STRUCTURAL CHEMISTRY

  • ISSN

    2053-2296

  • e-ISSN

  • Volume of the periodical

    75

  • Issue of the periodical within the volume

    JAN 2019

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    8

  • Pages from-to

    77-84

  • UT code for WoS article

    000454742800012

  • EID of the result in the Scopus database

    2-s2.0-85059295399