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Determination of 8-hydroxy-2 '-deoxyguanosine in urine with "linear" mode sparked graphite screen-printed electrodes

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216224%3A14310%2F21%3A00122813" target="_blank" >RIV/00216224:14310/21:00122813 - isvavai.cz</a>

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S0013468621016613?via%3Dihub" target="_blank" >https://www.sciencedirect.com/science/article/pii/S0013468621016613?via%3Dihub</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.electacta.2021.139371" target="_blank" >10.1016/j.electacta.2021.139371</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Determination of 8-hydroxy-2 '-deoxyguanosine in urine with "linear" mode sparked graphite screen-printed electrodes

  • Original language description

    The development of sensors for diagnostic purposes is of immense importance. Despite the number of proposed sensors showing attractive detection capabilities, the widespread use of these sensors is mainly hindered by selectivity issues and the elaborate tailoring of the sensing surface that eventually increases both the cost of the final sensor and the individual analysis cost. Herein, we report on the development of an advanced sensor for 8−hydroxy−2ˊ−deoxyguanosine (8−OHdG), an important biomarker for DNA oxidative damage. The sensor was developed on a low-cost graphite screen-printed electrode (SPE) by employing for the first time, an extremely fast SPE-to-graphite “linear” mode sparking process that enables the uniform modification of the whole electrode surface in less than 20 s. Graphite-sparked SPEs exhibited a linear relationship with the concentration of 8−OHdG over the range 2–50 nM, while the limit of detection (3σ) was 0.35 nM. The sensors showed a notable resistance to interference by 1000-fold excess of dopamine and ascorbic acid, and 100-fold excess of uric acid. A simple treatment of the samples, based on uricase, that eliminates the interference caused by uric acid under real-world conditions (&gt;1000-fold excess) was optimized and proposed. The method was successfully applied to the determination of 8−OHdG in synthetic urine samples. Recovery was 95%.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10405 - Electrochemistry (dry cells, batteries, fuel cells, corrosion metals, electrolysis)

Result continuities

  • Project

  • Continuities

    S - Specificky vyzkum na vysokych skolach<br>I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2021

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Electrochimica Acta

  • ISSN

    0013-4686

  • e-ISSN

    1873-3859

  • Volume of the periodical

    399

  • Issue of the periodical within the volume

    December

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    9

  • Pages from-to

    1-9

  • UT code for WoS article

    000711318400001

  • EID of the result in the Scopus database

    2-s2.0-85117086414