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Understanding the methyl-TROSY effect over a wide range of magnetic fields

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216224%3A14740%2F19%3A00110669" target="_blank" >RIV/00216224:14740/19:00110669 - isvavai.cz</a>

  • Result on the web

    <a href="https://aip.scitation.org/doi/10.1063/1.5095757" target="_blank" >https://aip.scitation.org/doi/10.1063/1.5095757</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1063/1.5095757" target="_blank" >10.1063/1.5095757</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Understanding the methyl-TROSY effect over a wide range of magnetic fields

  • Original language description

    The use of relaxation interference in the methyl Transverse Relaxation-Optimized SpectroscopY (TROSY) experiment has opened new avenues for the study of large proteins and protein assemblies in nuclear magnetic resonance. So far, the theoretical description of the methyl-TROSY experiment has been limited to the slow-tumbling approximation, which is correct for large proteins on high-field spectrometers. In a recent paper, favorable relaxation interference was observed in the methyl groups of a small protein at a magnetic field as low as 0.33 T, well outside the slow-tumbling regime. Here, we present a model to describe relaxation interference in methyl groups over a broad range of magnetic fields, not limited to the slow-tumbling regime. We predict that the type of multiple-quantum transition that shows favorable relaxation properties change with the magnetic field. Under the condition of fast methyl-group rotation, methyl-TROSY experiments can be recorded over the entire range of magnetic fields from a fraction of 1 T up to 100 T.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Chemical Physics

  • ISSN

    0021-9606

  • e-ISSN

  • Volume of the periodical

    150

  • Issue of the periodical within the volume

    22

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    12

  • Pages from-to

    224202

  • UT code for WoS article

    000471692400018

  • EID of the result in the Scopus database

    2-s2.0-85067360021