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Initial stage of physical ageing in network glasses

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F12%3A39895961" target="_blank" >RIV/00216275:25310/12:39895961 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1080/14786435.2012.704428" target="_blank" >http://dx.doi.org/10.1080/14786435.2012.704428</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1080/14786435.2012.704428" target="_blank" >10.1080/14786435.2012.704428</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Initial stage of physical ageing in network glasses

  • Original language description

    An atomistic view on Johari-Goldstein secondary beta-relaxation processes responsible for structural relaxation far below the glass transition temperature (T-g) in network glasses is developed for the archetypal chalcogenide glass, As20Se80, using positron annihilation lifetime, differential scanning calorimetry, Raman scattering and nuclear magnetic resonance techniques. Increased density fluctuations are shown to be responsible for the initial stage of physical ageing in these materials at the temperatures below T-g. They are correlated with changes in thermodynamic parameters of structural relaxation through the glass-to-supercooled liquid transition interval. General shrinkage, occurred during the next stage of physical ageing, is shown to be determined by the ability of system to release these redundant open volumes from the glass bulk through the densification process of glass network.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CA - Inorganic chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GAP204%2F11%2F0832" target="_blank" >GAP204/11/0832: Fabrication of optical elements based on micro- and nanostructuring of chalcogenide layers</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2012

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Philosophical Magazine

  • ISSN

    1478-6435

  • e-ISSN

  • Volume of the periodical

    92

  • Issue of the periodical within the volume

    33

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    12

  • Pages from-to

    4182-4193

  • UT code for WoS article

    000310854700009

  • EID of the result in the Scopus database