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Coordination of extraframework Li+ cation in the MCM-22 and MCM-36 zeolite: FTIR study of CO adsorbed

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F13%3A39896338" target="_blank" >RIV/00216275:25310/13:39896338 - isvavai.cz</a>

  • Alternative codes found

    RIV/61388955:_____/13:00391666

  • Result on the web

    <a href="http://link.springer.com/article/10.1007%2Fs10450-012-9467-2" target="_blank" >http://link.springer.com/article/10.1007%2Fs10450-012-9467-2</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s10450-012-9467-2" target="_blank" >10.1007/s10450-012-9467-2</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Coordination of extraframework Li+ cation in the MCM-22 and MCM-36 zeolite: FTIR study of CO adsorbed

  • Original language description

    Nature and population of Li+ cationic sites in MCM-22 zeolite and its pillared form (MCM-36) were investigated by means of adsorption of CO as a probe molecule. CO stretching frequency and adsorption heat were measured by FTIR spectroscopy and adsorptionmicrocalorimetry. Intrazeolitic carbonyl complexes on Li+ cations in MCM-22 and MCM-36 are characterized by two main vibrational bands at 2,195 and 2,188 cm(-1). Band at higher wavenumbers is ascribed to carbonyls on Li+ ions coordinated only to two oxygen atoms at the intersection of 10-ring channels and interacting with CO molecule by energy around 45 kJ mol(-1). Band at 2,188 cm(-1) was assigned to the carbonyls on Li+ cations located on top of 5 or 6-rings on the channel walls and coordinated to three or four oxygen atoms, interacting with CO molecule by energy 33-36 kJ mol(-1). Effect of pillaring and layered form of zeolite on nature and population of Li+ cationic sites is also discussed, as well as the formation of dicarbonyl co

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GBP106%2F12%2FG015" target="_blank" >GBP106/12/G015: Intelligent design of nanoporous adsorbents and catalysts</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2013

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Adsorption - Journal of the International Adsorption Society

  • ISSN

    0929-5607

  • e-ISSN

  • Volume of the periodical

    19

  • Issue of the periodical within the volume

    2-4

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    9

  • Pages from-to

    455-463

  • UT code for WoS article

    000317620800027

  • EID of the result in the Scopus database