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The effect of molecular structure on thermal stability, decomposition kinetics and reaction models of nitric esters

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F13%3A39896350" target="_blank" >RIV/00216275:25310/13:39896350 - isvavai.cz</a>

  • Result on the web

    <a href="http://www.sciencedirect.com/science/article/pii/S0040603113002931" target="_blank" >http://www.sciencedirect.com/science/article/pii/S0040603113002931</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.tca.2013.05.032" target="_blank" >10.1016/j.tca.2013.05.032</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    The effect of molecular structure on thermal stability, decomposition kinetics and reaction models of nitric esters

  • Original language description

    The thermal stability and decompn. mechanism functions of 10 nitric esters including nitroglycerin (NG), pentaerythritol tetranitrate (PETN), trimethylolethane trinitrate (TMETN), dipentaerythritol hexanitrate (DiPEHN), trimethylolpropane trinitrate (TMPTN), erythritol tetranitrate (ETN), xylitol pentanitrate (XPN), sorbitol hexanitrate (SHN), mannitol hexanitrate (MHN), and nitroisobutylglycerol trinitrate (NIBGT) are detd. by non-isothermal TG and DSC techniques. It was found that the mean activationenergies for most nitric esters are comparable at const. heating rate (around 145 kJ mol-1), indicating that their main decompn. pathways might be the same. Based on the crit. temp. of thermal decompn., the order of mol. stability for involved nitric esters is found to be MHN { XPN { TMPTN { SHN { NIBGT { ETN { PETN { DiPEHN. The introduction of function groups to the tertiary carbon is in favor of increasing thermal stability due to increase of symmetry and rigidity of the mol.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/VG20102014032" target="_blank" >VG20102014032: Research of improvised explosives detection by dogs</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2013

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Thermochimica Acta

  • ISSN

    0040-6031

  • e-ISSN

  • Volume of the periodical

    566

  • Issue of the periodical within the volume

    N

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    12

  • Pages from-to

    137-148

  • UT code for WoS article

    000322685700020

  • EID of the result in the Scopus database