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Methane adsorption in ADOR zeolites: a combined experimental and DFT/CC study

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F17%3A39911948" target="_blank" >RIV/00216275:25310/17:39911948 - isvavai.cz</a>

  • Alternative codes found

    RIV/61388955:_____/17:00477446 RIV/61388963:_____/17:00477446

  • Result on the web

    <a href="http://dx.doi.org/10.1039/c7cp02315d" target="_blank" >http://dx.doi.org/10.1039/c7cp02315d</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1039/c7cp02315d" target="_blank" >10.1039/c7cp02315d</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Methane adsorption in ADOR zeolites: a combined experimental and DFT/CC study

  • Original language description

    Physical adsorption of methane in purely siliceous molecular sieves prepared by a recently discovered synthetic pathway using 2D zeolites as nanoscale building blocks has been investigated by means of combined experimental and theoretical approaches. The DFT/CC-based method has been tested on ADOR zeolites of the UTL family and a few experimentally well-characterized siliceous zeolites. Excellent agreement between theoretical and experimental heats of adsorption has been found for OKO, PCR, MFI, CHA and AEI zeolites. The observed discrepancy for the UTL germanosilicate (2 kJ mol(-1)) has been plausibly explained using a simple model of D4R defects. The proposed methodology can be used as a reliable characterization tool for newly synthesized silica nanomaterials.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Physical Chemistry Chemical Physics

  • ISSN

    1463-9076

  • e-ISSN

  • Volume of the periodical

    19

  • Issue of the periodical within the volume

    25

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    8

  • Pages from-to

    16533-16540

  • UT code for WoS article

    000404530600026

  • EID of the result in the Scopus database

    2-s2.0-85021981835