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FeOx/Al2O3 Catalysts for High-temperature Decomposition of N2O Under Conditions of NH3 Oxidation in Nitric Acid Production

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F18%3A39913130" target="_blank" >RIV/00216275:25310/18:39913130 - isvavai.cz</a>

  • Alternative codes found

    RIV/61388955:_____/18:00490607 RIV/00216208:11320/18:10378480 RIV/60461373:22310/18:43915957

  • Result on the web

    <a href="http://dx.doi.org/10.1039/c8cy00383a" target="_blank" >http://dx.doi.org/10.1039/c8cy00383a</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1039/c8cy00383a" target="_blank" >10.1039/c8cy00383a</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    FeOx/Al2O3 Catalysts for High-temperature Decomposition of N2O Under Conditions of NH3 Oxidation in Nitric Acid Production

  • Original language description

    The catalytic activity of a series of FeOx/Al2O3 prepared under various conditions was evaluated for high temperature decomposition of N2O (HT-deN(2)O) in a complex gas mixture produced by oxidation of ammonia. Thus the relevant step in the industrial nitric acid production process was simulated. The catalyst stability during long-term exposure (12 days) to reaction conditions relevant to HT-deN(2)O was studied. Both fresh and aged FeOx/Al2O3 exhibited more than 90% conversion of N2O in the 750-900 degrees C temperature range. Structural analysis showed that the prepared FeOx/Al2O3 catalysts contained various proportions of , and alumina phases and up to four individual iron species. In the and Al2O3 phases, well stabilized Fe(iii) in T-d or O-h coordination was identified as the active species in HT-deN(2)O.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2018

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Catalysis Science and Technology

  • ISSN

    2044-4753

  • e-ISSN

  • Volume of the periodical

    8

  • Issue of the periodical within the volume

    11

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    12

  • Pages from-to

    2841-2852

  • UT code for WoS article

    000434386000011

  • EID of the result in the Scopus database

    2-s2.0-85048257095