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Effective Performance Modifications for a Composite Rocket Propellant via Coagglomerates of Cyclic Nitramines

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F25%3A39922835" target="_blank" >RIV/00216275:25310/25:39922835 - isvavai.cz</a>

  • Result on the web

    <a href="https://doi.org/10.1021/acsomega.5c01848" target="_blank" >https://doi.org/10.1021/acsomega.5c01848</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acsomega.5c01848" target="_blank" >10.1021/acsomega.5c01848</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Effective Performance Modifications for a Composite Rocket Propellant via Coagglomerates of Cyclic Nitramines

  • Original language description

    The new combustion modifier cis-1,3,4,6-tetranitrooctahydroimidazo-[4,5-d]imidazole (BCHMX) was tested on an aluminum HMX/HTPB/AP propellant. Monitored were the changes in the propellant characteristics, when the 10, 20, and 30 wt % ammonium perchlorate (AP) were substituted by pure 1,3,5,7-tetranitro-1,3,5.7-tetrazocane (HMX), mechanical mixture HMX/BCHMX (PM), and coagglomerate of HMX/BCHMX (CACs), the latter two in a weight ratio of 8:1. By means of the powder X-ray diffraction and FTIR and Raman spectroscopies, it was confirmed that CACs are a mixture of cocrystal βHMX/BCHMX with excess β-HMX. The relationships were discovered between the burning rate of the prepared samples and the heat of combustion (Qc), ignition temperature, specific rate constant of thermal decomposition, impact sensitivity, hardness, and specific impulse. Correspondingly, relationships between Qc and ignition temperature, as well as the impact and friction sensitivities, were investigated. It was found that increasing the amount of CACs n the propellant reduces the pressure exponent, while pure HMX and PM have the opposite effect. The significantly positive effectof CACs on the burning rate, especially at 20 wt % substitution of AP by these microcrystals, is another noteworthy finding.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20505 - Composites (including laminates, reinforced plastics, cermets, combined natural and synthetic fibre fabrics; filled composites)

Result continuities

  • Project

  • Continuities

    S - Specificky vyzkum na vysokych skolach<br>I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2025

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    ACS Omega

  • ISSN

    2470-1343

  • e-ISSN

    2470-1343

  • Volume of the periodical

    10

  • Issue of the periodical within the volume

    27

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    15

  • Pages from-to

    29194-29208

  • UT code for WoS article

    001498236600001

  • EID of the result in the Scopus database

    2-s2.0-105006787162