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Advanced space-charge-limited current model for analyzing fermi level shift in the bandgap of halide perovskites

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26310%2F26%3A0198537" target="_blank" >RIV/00216305:26310/26:0198537 - isvavai.cz</a>

  • Result on the web

    <a href="https://www.nature.com/articles/s42005-025-02202-1" target="_blank" >https://www.nature.com/articles/s42005-025-02202-1</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1038/s42005-025-02202-1" target="_blank" >10.1038/s42005-025-02202-1</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Advanced space-charge-limited current model for analyzing fermi level shift in the bandgap of halide perovskites

  • Original language description

    Understanding how charge carriers behave in semiconductors is key to improving next-generation optoelectronic devices. Here we introduce an advanced space-charge-limited current model that enables detailed extraction of mobility, charge carrier concentrations, and Fermi level position from voltage- and energy-dependent analysis. Applying this model to two promising halide perovskites, methylammonium lead bromide and methylammonium lead iodide, we observe a strong photoresponse, with significant increases in microscopic mobility and free carrier density under illumination. Interestingly, the behavior of trapped charges and Fermi level shifts differs between the two materials, revealing distinct transport mechanisms. This model offers a powerful tool for characterizing semiconductors and could accelerate the development of more efficient light-sensitive devices.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10300 - Physical sciences

Result continuities

  • Project

    <a href="/en/project/GA25-17500S" target="_blank" >GA25-17500S: Tunable perovskite metasurfaces for a new generation of optical quantum technologies</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2025

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Communications Physics

  • ISSN

  • e-ISSN

    2399-3650

  • Volume of the periodical

    8

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    10

  • Pages from-to

    1-10

  • UT code for WoS article

    001523035700001

  • EID of the result in the Scopus database