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Biodegradation of polyurethane‐polyhydroxybutyrate elastomeric composite investigated from morphological and structural viewpoint

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26620%2F19%3APU128971" target="_blank" >RIV/00216305:26620/19:PU128971 - isvavai.cz</a>

  • Result on the web

    <a href="https://onlinelibrary.wiley.com/doi/full/10.1002/app.46909" target="_blank" >https://onlinelibrary.wiley.com/doi/full/10.1002/app.46909</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/app.46909" target="_blank" >10.1002/app.46909</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Biodegradation of polyurethane‐polyhydroxybutyrate elastomeric composite investigated from morphological and structural viewpoint

  • Original language description

    Morphological, structural, and tensile changes of polyurethane‐poly(3‐hydroxybutyrate) (PU‐PHB) elastomeric composites were evaluated after accelerated test in standard compost media. Size of PHB particles together with their uniform dispersion in the matrix were found to be key parameters for material's resistivity against degradation media. PU‐PHB composite films were synthesized by the “green” solvent free method, where commercially available PHB (PHB‐COM) and PHB produced by bacterium Cupriavidus necator H16 (PHB‐BUT) were both used in the amount of 1, 5, and 10 wt % in composites. Scanning electron microscopy revealed excellent dispersion of PHB‐COM microparticles in the PU matrix resulting in negligible weight losses of the material (max 0.7 wt %). On the contrary, PHB‐BUT particles were agglomerated which promoted partial degradation of the material (max 3.3 wt % loss) manifested by holes on the surface but without severe damage (e.g. fragmentation). Structural analysis confirmed lower crystallinity and less ordered crystalline phase of PHB after the degradation test, particularly in composites made of PHB‐BUT. Moreover, the materials were less stiff after the composting test, but beneficial with higher elongation at break. Such properties are favorable for the use of renewable PHB in the current industrial applications of PU elastomers. (c) 2018 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2018, 135, 46909.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10404 - Polymer science

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Applied Polymer Sciences

  • ISSN

    0021-8995

  • e-ISSN

    1097-4628

  • Volume of the periodical

    136

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    8

  • Pages from-to

    „46909-1“-„46909-8“

  • UT code for WoS article

    000450307600011

  • EID of the result in the Scopus database

    2-s2.0-85052473529