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Effect of substitutional oxygen on the cohesion of transition-metal nitride multilayers

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26620%2F23%3APU148527" target="_blank" >RIV/00216305:26620/23:PU148527 - isvavai.cz</a>

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S0257897223003584?via%3Dihub" target="_blank" >https://www.sciencedirect.com/science/article/pii/S0257897223003584?via%3Dihub</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.surfcoat.2023.129583" target="_blank" >10.1016/j.surfcoat.2023.129583</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Effect of substitutional oxygen on the cohesion of transition-metal nitride multilayers

  • Original language description

    Using a first-principles approach, we investigated the effect of oxygen as a substitutional impurity on cohesion of three transition metal nitride multilayers. Namely, we studied AlN/VN, AlN/TiN, and VN/TiN systems in a rock salt structure (B1) with (0 0 1) interfaces. The preferred oxygen positions were determined with the help of calculations of free energy that also included contribution from the vibrational entropy. Subsequent calculations of the cleavage energy for all possible cleavage planes enabled us to identify the weakest link and assess the impact of the oxygen impurity on a cohesion of each of the studied multilayers. Supercells of different sizes were used to estimate the effect of oxygen concentration. Our results indicate that oxygen prefers to replace nitrogen atoms in interfacial planes and that these impurities do not reduce the multilayer cohesion. Moreover, in the case of the AlN/TiN system, their presence was found to increase cohesion of the interface.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20501 - Materials engineering

Result continuities

  • Project

    <a href="/en/project/GA20-08130S" target="_blank" >GA20-08130S: Role of Entropy in Materials Science: Grain Boundary Segregation</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Surface and Coatings Technology

  • ISSN

    0257-8972

  • e-ISSN

  • Volume of the periodical

    465

  • Issue of the periodical within the volume

    7

  • Country of publishing house

    CH - SWITZERLAND

  • Number of pages

    7

  • Pages from-to

    „129583“-„“

  • UT code for WoS article

    001009858900001

  • EID of the result in the Scopus database

    2-s2.0-85156230204