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Variation of Spin-Transition Temperature in the Iron(III) Complex Induced by Different Compositions of the Crystallization Solvent

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26620%2F23%3APU148623" target="_blank" >RIV/00216305:26620/23:PU148623 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989592:15310/23:73621967

  • Result on the web

    <a href="https://pubs.acs.org/doi/10.1021/acs.cgd.2c01411" target="_blank" >https://pubs.acs.org/doi/10.1021/acs.cgd.2c01411</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.cgd.2c01411" target="_blank" >10.1021/acs.cgd.2c01411</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Variation of Spin-Transition Temperature in the Iron(III) Complex Induced by Different Compositions of the Crystallization Solvent

  • Original language description

    We crystallized the Schiff-base iron(III) spin-crossover complex [Fe(3,5Cl-L5)(NCSe)] from different two-component solvent mixtures containing methanol and chloroform (phi = V(CH3OH)/V(solvent) = 0.05, 0.25, 0.50, 0.83, and 1.00). The obtained crystalline products were characterized by X-ray diffraction, and it was confirmed that they are all composed of the same crystalline phase, and they do not contain any crystal solvent. However, significant differences in magnetic properties were observed, and thermal hysteresis changed from (in K) 121T down arrow and 134T up arrow for phi = 0.05 and 0.25, down to 72T down arrow and 96T up arrow for phi = 1.00. The crystal structures of the low-spin and high-spin phases were studied theoretically and experimentally.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

  • Continuities

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Crystal Growth and Design

  • ISSN

    1528-7483

  • e-ISSN

    1528-7505

  • Volume of the periodical

    23

  • Issue of the periodical within the volume

    3

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    7

  • Pages from-to

    1323-1329

  • UT code for WoS article

    000934881600001

  • EID of the result in the Scopus database

    2-s2.0-85148663549