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Ultrafast laser-induced spin-lattice dynamics in the van der Waals antiferromagnet CoPS3

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26620%2F23%3APU149098" target="_blank" >RIV/00216305:26620/23:PU149098 - isvavai.cz</a>

  • Result on the web

    <a href="https://pubs.aip.org/aip/apm/article/11/7/071104/2900821/Ultrafast-laser-induced-spin-lattice-dynamics-in" target="_blank" >https://pubs.aip.org/aip/apm/article/11/7/071104/2900821/Ultrafast-laser-induced-spin-lattice-dynamics-in</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1063/5.0146128" target="_blank" >10.1063/5.0146128</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Ultrafast laser-induced spin-lattice dynamics in the van der Waals antiferromagnet CoPS3

  • Original language description

    CoPS3 stands out in the family of the van der Waals antiferromagnets XPS3 (X = Mn, Ni, Fe, and Co) due to the unquenched orbital momentum of the magnetic Co2+ ions, which is known to facilitate the coupling of spins to both electromagnetic waves and lattice vibrations. Here, using a time-resolved magneto-optical pump-probe technique, we experimentally study the ultrafast laser-induced dynamics of mutually correlated spins and lattice. It is shown that a femtosecond laser pulse acts as an ultrafast heater and, thus, results in the melting of the antiferromagnetic order. At the same time, the resonant pumping of the T-4(1g) ? T-4(2g) electronic transition in Co2+ ions effectively changes their orbital momentum, giving rise to a mechanical force that moves the ions in the direction parallel to the orientation of their spins, thus generating a coherent B-g phonon mode at the frequency of about 4.7 THz.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    21002 - Nano-processes (applications on nano-scale); (biomaterials to be 2.9)

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    APL Materials

  • ISSN

    2166-532X

  • e-ISSN

  • Volume of the periodical

    11

  • Issue of the periodical within the volume

    7

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    9

  • Pages from-to

    „“-„“

  • UT code for WoS article

    001023585200005

  • EID of the result in the Scopus database

    2-s2.0-85164299881