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Oxidation Behavior and Outward Diffusion of Al Along Oxide Grain Boundaries of FeCrAl Alloys Overdoped with Zr and Hf

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26620%2F24%3APU150752" target="_blank" >RIV/00216305:26620/24:PU150752 - isvavai.cz</a>

  • Alternative codes found

    RIV/68081723:_____/24:00603683

  • Result on the web

    <a href="https://link.springer.com/article/10.1007/s11085-023-10204-z" target="_blank" >https://link.springer.com/article/10.1007/s11085-023-10204-z</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s11085-023-10204-z" target="_blank" >10.1007/s11085-023-10204-z</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Oxidation Behavior and Outward Diffusion of Al Along Oxide Grain Boundaries of FeCrAl Alloys Overdoped with Zr and Hf

  • Original language description

    The formation of the alpha-Al2O3 scale on reactive element (RE)-doped FeCrAl alloys is commonly believed to be primarily caused by inward oxygen transport along grain boundaries. However, this study suggests that metal ion outward diffusion also plays a role in the development of the oxide scales and their microstructural characteristics. The study examines the oxidation behavior and grain boundary outward diffusion of iron-chromium alloys containing similar to 10 at% aluminum and similar to 22 at% chromium, doped with an over-critical concentration of REs, i.e., Zr and Hf. All samples were investigated after thermal exposure at 1100 degrees C by scanning electron microscopy (SEM), transmission electron microscopy (TEM), and atom probe tomography (APT). As a result of the overdoping, a considerable increase in oxide growth, an increase in the depth of internal oxidation, and RE-oxide formation near and at oxide grain boundaries (GBs) were observed as a consequence of increased inward and outward diffusion. The effect of overdoping manifests itself differently depending on the RE type and amount due to different solubility, ionic size, and electronic structure of alumina. The sample with Zr retained the adhesion of alumina to the alloy after the first and second thermal exposure, while Hf overdoping resulted in severe spallation after the second thermal exposure.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20504 - Ceramics

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    HIGH TEMPERATURE CORROSION OF MATERIALS

  • ISSN

    2731-8397

  • e-ISSN

  • Volume of the periodical

    101

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    19

  • Pages from-to

    41-59

  • UT code for WoS article

    001094155200002

  • EID of the result in the Scopus database

    2-s2.0-85175324759