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Comparison of sorbents for caesium removal from aqueous environment

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F26722445%3A_____%2F18%3AN0000103" target="_blank" >RIV/26722445:_____/18:N0000103 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Comparison of sorbents for caesium removal from aqueous environment

  • Original language description

    This study compares the sorbent effectiveness of a caesium removal from water solutions. Caesium, namely the 137Cs isotope, is a fission product of uranium (235U) breakdown. The isotope 137Cs with the half-life decay of 30 years is an undesirable contaminant in a primary coolant of nuclear power plant. The 137Cs isotope is main contributor to overall radioactivity in a reactor coolant. Caesium leaks in the coolant water of a primary circuit trough microcracks in fuel rods. Damage of fuel rods is quite common, but usually less than 0,02 % per a reactor campaign. Caesium in the technological water needs to be removed due to high radioactivity. This work compares two zeolite materials and their ability to remove caesium from aqueous solution. Zeolites are, in general, hydrated aluminosilicate materials that behave as cation exchangers. They are able to exchange cations from an aqueous solution for cations located on their surface, particularly for Na+ , K+ , Mg2+ and Ca2+. A natural zeolite and its modified form with the high content of clinoptilolite were used for sorption experiments. The modification was performed using Co(NO3)2 and K4[Fe(CN)6] in order to form K2Co[Fe(CN)6] on a zeolite surface. Zeolites were characterized by an infrared and Raman Spectroscopy, SEM, and BET surface area measurement. Sorption experiments were conducted in a batch arrangement. The optimum pH for sorption and parameters of Langmuir isotherm were determined. The influence of accompanying monovalent and divalent cations on the sorption of caesium was observed.

  • Czech name

  • Czech description

Classification

  • Type

    D - Article in proceedings

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2018

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    Proceedings of the 6 th International Conference on Chemical Technology

  • ISBN

    978-80-86238-77-7

  • ISSN

  • e-ISSN

  • Number of pages

    6

  • Pages from-to

    436-442

  • Publisher name

    Česká společnost průmyslové chemie

  • Place of publication

    Praha

  • Event location

    Mikulov

  • Event date

    Apr 16, 2018

  • Type of event by nationality

    EUR - Evropská akce

  • UT code for WoS article