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Comparative modeling of an in situ diffusion experiment in granite at the Grimsel Test Site

Result description

An in situ diffusion experiment was performed at the Grimsel Test Site (Switzerland). Several tracers (H-3 as HTO, Na-22(+), Cs-134(+), I-131(-) with stable I- as carrier) were continuously circulated through a packed-off borehole and the decrease in tracer concentrations in the liquid phase was monitored for a period of about 2 years. Subsequently, the borehole section was overcored and the tracer profiles in the rock analyzed (H-3, Na-22(+), Cs-134(+)) H-3 and Na-22(+) showed a similar decrease in activity in the circulation system (slightly larger drop for H-3). The drop in activity for Cs-134(+) was much more pronounced. Transport distances in the rock were about 20 cm for H-3, 10 cm for Na-22(+), and 1 cm for Cs-134(+). The dataset (except for I-131(-) because of complete decay at the end of the experiment) was analyzed with different diffusion-sorption models by different teams (IDAEA-CSIC, UJV-Rez, JAEA) using different codes, with the goal of obtaining effective diffusion coefficients (D-e) and porosity (phi) or rock capacity (alpha) values.

Keywords

GrimselDiffusionGraniteModeling

The result's identifiers

Alternative languages

  • Result language

    angličtina

  • Original language name

    Comparative modeling of an in situ diffusion experiment in granite at the Grimsel Test Site

  • Original language description

    An in situ diffusion experiment was performed at the Grimsel Test Site (Switzerland). Several tracers (H-3 as HTO, Na-22(+), Cs-134(+), I-131(-) with stable I- as carrier) were continuously circulated through a packed-off borehole and the decrease in tracer concentrations in the liquid phase was monitored for a period of about 2 years. Subsequently, the borehole section was overcored and the tracer profiles in the rock analyzed (H-3, Na-22(+), Cs-134(+)) H-3 and Na-22(+) showed a similar decrease in activity in the circulation system (slightly larger drop for H-3). The drop in activity for Cs-134(+) was much more pronounced. Transport distances in the rock were about 20 cm for H-3, 10 cm for Na-22(+), and 1 cm for Cs-134(+). The dataset (except for I-131(-) because of complete decay at the end of the experiment) was analyzed with different diffusion-sorption models by different teams (IDAEA-CSIC, UJV-Rez, JAEA) using different codes, with the goal of obtaining effective diffusion coefficients (D-e) and porosity (phi) or rock capacity (alpha) values.

  • Czech name

  • Czech description

Classification

  • Type

    Jx - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    DL - Nuclear waste, radioactive pollution and control

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    V - Vyzkumna aktivita podporovana z jinych verejnych zdroju

Others

  • Publication year

    2015

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Contaminant Hydrology

  • ISSN

    0169-7722

  • e-ISSN

  • Volume of the periodical

    179

  • Issue of the periodical within the volume

    August

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    13

  • Pages from-to

    89-101

  • UT code for WoS article

  • EID of the result in the Scopus database