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Magnetic and electronic properties of Neptunium chalcogenides from GGA U SOC and DFT investigations

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F49777513%3A23640%2F17%3A43932211" target="_blank" >RIV/49777513:23640/17:43932211 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.jmmm.2017.01.073" target="_blank" >http://dx.doi.org/10.1016/j.jmmm.2017.01.073</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.jmmm.2017.01.073" target="_blank" >10.1016/j.jmmm.2017.01.073</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Magnetic and electronic properties of Neptunium chalcogenides from GGA U SOC and DFT investigations

  • Original language description

    First-principles calculations techniques were employed to explore the structural, electronic and magnetic properties of Neptunium chalcogenides (Np2X5, X = S, Se and Te). No experimental or theoretical studies of their physical properties have been previously reported in the literature. The presence of highly localized f states has requested the employment of the spin orbit coupling and GGA + U approach in order to describe correctly the f–f coupling. Np2X5 was found metallic with high magnetic character due to the Neptunium presence. Fermi surfaces of Np2Te5 have shown a greater electrical conductivity compared to Np2Se5 and Np2S5. The magnetic moment was found to be between 13.24 and 13.92 μB, principally induced by Np f and d-orbitals as well as the spin-polarization of the chalcogenes (Te, Se, S) induced by Np. Neptunium chalcogenides have shown interesting magnetic properties and should be manipulated with precaution due to their radioactive properties.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10301 - Atomic, molecular and chemical physics (physics of atoms and molecules including collision, interaction with radiation, magnetic resonances, Mössbauer effect)

Result continuities

  • Project

  • Continuities

    O - Projekt operacniho programu

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS

  • ISSN

    0304-8853

  • e-ISSN

  • Volume of the periodical

    432

  • Issue of the periodical within the volume

    JUN 15 2017

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    7

  • Pages from-to

    574-580

  • UT code for WoS article

    000399601600086

  • EID of the result in the Scopus database

    2-s2.0-85015329477