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Calculations of 19F NMR shieldings in polyfluoro-1-lithioethenes: Role of geometry, solvation and comparison with experimental shifts

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F02%3A00006493" target="_blank" >RIV/60461373:22310/02:00006493 - isvavai.cz</a>

  • Alternative codes found

    RIV/61389013:_____/02:55033160

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Calculations of 19F NMR shieldings in polyfluoro-1-lithioethenes: Role of geometry, solvation and comparison with experimental shifts

  • Original language description

    19F NMR chemical shielding constants in (E)-1,2-difluoroethenyllithium (1) and trifluoroethenyllithium (2) have been calculated by the SOS-DFPT-IGLO1 method and employed for an assignment of individual signals in experimental 19F NMR spectra of polyfluoro-1-lithioethenes. The role of solvation on equilibrium geometries and consequently on the shielding constants is discussed. In comparison to HF2 or MP2 methods, DFT calculated absolute shielding values for fluoroalkenes differ from the experimental values by an opposite offset error. All methods gave acceptable relative shielding values.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CC - Organic chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA203%2F99%2F1630" target="_blank" >GA203/99/1630: 1-fluoro-1-lithioalkanes and 1-fluoro-1lithio-1-alkanes - synthesis, stability study and synthetic applications</a><br>

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2002

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Fluorine Chemistry

  • ISSN

    0022-1139

  • e-ISSN

  • Volume of the periodical

    116

  • Issue of the periodical within the volume

    2

  • Country of publishing house

    BE - BELGIUM

  • Number of pages

    7

  • Pages from-to

    121-127

  • UT code for WoS article

  • EID of the result in the Scopus database