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Plasmon-Assisted Activation and Grafting by Iodonium Salt: Functionalization of Optical Fiber Surface

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F18%3A43916315" target="_blank" >RIV/60461373:22310/18:43916315 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1002/admi.201800725" target="_blank" >http://dx.doi.org/10.1002/admi.201800725</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/admi.201800725" target="_blank" >10.1002/admi.201800725</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Plasmon-Assisted Activation and Grafting by Iodonium Salt: Functionalization of Optical Fiber Surface

  • Original language description

    In this paper, the utilization of plasmon-induced cleavage of CI bond in the structure of iodonium salt followed by grafting of organic radicals to Au surface is proposed. The plasmon is excited by the coupling of Au-covered optical fiber with the laser light source, with wavelength corresponding to the plasmon absorption band, and immersion of fiber in the solution of iodonium salt. Grafting procedure is monitored through the shift of surface plasmon resonanse (SPR) position during the laser light transmission. Further verifications are performed using the surface enhanced Raman spectroscopy (SERS) and scanning electron microscopy and energy-dispersive X-ray spectroscopy methods. Only in the case of coincidence of coupled laser emission and initial SPR absorption band wavelengths efficient activation of diaryliodonium salt (IS) is observed. With the aim to introduce hydrophobic and repellent surface properties the di-[3,5-bis(trifluoromethyl)phenyl]iodonium tetrafluoroborate salt is used. Surface functionality is further tested using the wettability and antifouling test. Proposed method for the first time utilizes the plasmonic phenomenon as an effective tool for initiating the iodonium salt heterophase reaction and can be considered as extremely effective approach in the case of surface activation, in terms of energy and materials harvesting.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20501 - Materials engineering

Result continuities

  • Project

    <a href="/en/project/NV15-33459A" target="_blank" >NV15-33459A: Biomedical photonic devices for advanced medicinal diagnostics and therapy</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2018

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Advanced Materials Interfaces

  • ISSN

    2196-7350

  • e-ISSN

  • Volume of the periodical

    5

  • Issue of the periodical within the volume

    20

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    8

  • Pages from-to

    "1800725/1"-8

  • UT code for WoS article

    000448787800006

  • EID of the result in the Scopus database