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Structure determination of butylone as a new psychoactivesubstance using chiroptical and vibrational spectroscopies

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F18%3A43916406" target="_blank" >RIV/60461373:22310/18:43916406 - isvavai.cz</a>

  • Alternative codes found

    RIV/60461373:22330/18:43916406 RIV/60461373:22340/18:43916406 RIV/60461373:22810/18:43916406

  • Result on the web

    <a href="https://onlinelibrary.wiley.com/doi/epdf/10.1002/chir.22825" target="_blank" >https://onlinelibrary.wiley.com/doi/epdf/10.1002/chir.22825</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/chir.22825" target="_blank" >10.1002/chir.22825</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Structure determination of butylone as a new psychoactivesubstance using chiroptical and vibrational spectroscopies

  • Original language description

    Recently, there has been a worldwide substantial increase in the consumptionof new psychoactive substances (NPS), compounds that mimic the structureof illicit drugs, such as amphetamines or ecstasy. The producers try to avoidthe law by a slight modification of illicit structures, thereby developing dozensof temporarily legal NPS every year. The current trends in the detection andmonitoring of such substances demand a fast and reliable analysis. Molecularspectroscopy represents a highly effective tool for the identification of NPSand chiroptical methods can provide further information on their 3D structure,which is the key for the determination of their biological activity. We presentthe first systematic study of NPS, specifically butylone, combining chiropticaland vibrational spectroscopies withab initiocalculations. According to densityfunctional theory calculations, 6 stable lowest energy conformers of butylonewere found and their molecular structure was described. For each conformer,the relative abundance based on the Boltzmann distribution was estimated,their population weighted spectra predicted and compared to the experimentalresults. Very good agreement between the experimental and the simulatedspectra was achieved, which allowed not only the assignment of the absoluteconfiguration, but also a precise description of the molecular structure.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10406 - Analytical chemistry

Result continuities

  • Project

    <a href="/en/project/LO1601" target="_blank" >LO1601: Prague University Analytical Centre II and III - NPU 2015-2020</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>S - Specificky vyzkum na vysokych skolach<br>I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2018

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Chirality

  • ISSN

    0899-0042

  • e-ISSN

  • Volume of the periodical

    30

  • Issue of the periodical within the volume

    5

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    12

  • Pages from-to

    548-559

  • UT code for WoS article

    000430466200004

  • EID of the result in the Scopus database

    2-s2.0-85041713108