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Viscosity and configuration entropy of glasses for CHROMPIC vitrification

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F18%3A43917254" target="_blank" >RIV/60461373:22310/18:43917254 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1007/s10973-017-6652-2" target="_blank" >http://dx.doi.org/10.1007/s10973-017-6652-2</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s10973-017-6652-2" target="_blank" >10.1007/s10973-017-6652-2</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Viscosity and configuration entropy of glasses for CHROMPIC vitrification

  • Original language description

    The composition and temperature dependence of viscosity and configuration entropy of glasses with chemical composition close to that used for CHROMPIC radioactive waste vitrification were studied. The composition of fifteen studied glasses was derived from the composition of currently used glass frit by increasing/decreasing the content of each particular oxide and retaining the same relative amounts of the other components. The high-temperature viscosity in the range (10(1.8)-10(3.0)) dPa s was measured by the falling ball method while the low-temperature viscosity in the range (10(8)-10(12)) dPa s was measured by the thermomechanical analysis. The experimental viscosity data were smoothed by the Vogel-Fulcher-Tammann viscosity equation. The temperature-composition dependence of viscosity was described by the Adam and Gibbs viscosity equation. The influence of increasing/decreasing content of particular oxides on the values of parameters of the Adam and Gibbs viscosity equation and on the value of configuration entropy was quantified and discussed.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20504 - Ceramics

Result continuities

  • Project

  • Continuities

    S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2018

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Thermal Analysis and Calorimetry

  • ISSN

    1388-6150

  • e-ISSN

  • Volume of the periodical

    133

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    6

  • Pages from-to

    365-370

  • UT code for WoS article

    000435398700034

  • EID of the result in the Scopus database