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Reaction of lithiated thiophene-derived aminocarbene complexes with inorganic halides: Preparation of a heteroatom containing mono- and multicarbene complexes

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F19%3A43917260" target="_blank" >RIV/60461373:22310/19:43917260 - isvavai.cz</a>

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S0022328X18309355" target="_blank" >https://www.sciencedirect.com/science/article/pii/S0022328X18309355</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.jorganchem.2018.12.015" target="_blank" >10.1016/j.jorganchem.2018.12.015</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Reaction of lithiated thiophene-derived aminocarbene complexes with inorganic halides: Preparation of a heteroatom containing mono- and multicarbene complexes

  • Original language description

    The reaction of lithiated pentacarbonyl [(N,N-dimethylamino) (2-thienyl)carbene]chromium (0) or pentacarbonyl [(N,N-dimethylamino) (2-thienyl)carbene]tungsten (0) with SOCl2, COCl2, Me3 SiCl, Me2SiCl2, Me3SnCl and SnCl4 afforded the corresponding carbene complexes, in which the chlorine was substituted with a 2-thienyl amino carbene moiety. Reaction with S2Cl2 afforded the corresponding biscarbene sulphide. In contrast, reactions with the phosphorous chlorides PCl3, POCl3, PhPCl2 and Ph2PCl were unsuccessful. The trimethylstannyl derivative was successfully used in Stille coupling with 4- nitroiodobenzene. The molecular structure of the tungsten tetracarbene derived from SnCl4 was obtained.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10401 - Organic chemistry

Result continuities

  • Project

    <a href="/en/project/GA17-21770S" target="_blank" >GA17-21770S: Modular Synthesis of New Fischer Biscarbene Complexes, their Structural Features and Synthetic Applications</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Organometallic Chemistry

  • ISSN

    0022-328X

  • e-ISSN

  • Volume of the periodical

    882

  • Issue of the periodical within the volume

    leden

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    6

  • Pages from-to

    90-95

  • UT code for WoS article

    000456533700012

  • EID of the result in the Scopus database

    2-s2.0-85059760881