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Multifunctional Visible-Light Powered Micromotors Based on Semiconducting Sulfur- and Nitrogen-Containing Donor-Acceptor Polymer

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F20%3A43920514" target="_blank" >RIV/60461373:22310/20:43920514 - isvavai.cz</a>

  • Alternative codes found

    RIV/00216305:26620/20:PU138044

  • Result on the web

    <a href="https://onlinelibrary.wiley.com/doi/full/10.1002/adfm.202002701" target="_blank" >https://onlinelibrary.wiley.com/doi/full/10.1002/adfm.202002701</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/adfm.202002701" target="_blank" >10.1002/adfm.202002701</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Multifunctional Visible-Light Powered Micromotors Based on Semiconducting Sulfur- and Nitrogen-Containing Donor-Acceptor Polymer

  • Original language description

    Photosensitive micromotors that can be remotely controlled by visible light irradiation demonstrate great potential in biomedical and environmental applications. To date, a vast number of light-driven micromotors are mainly composed from costly heavy and precious metal-containing multicomponent systems, that limit the modularity of chemical and physical properties of these materials. Herein, a highly efficient photocatalytic micromotors based exclusively on a purely organic polymer framework-semiconducting sulfur- and nitrogen-containing donor-acceptor polymer, is presented. Thanks to precisely tuned molecular architecture, this material has the ability to absorb visible light due to a conveniently situated energy gap. In addition, the donor-acceptor dyads within the polymer backbone ensure efficient photoexcited charge separation. Hence, these polymer-based micromotors can move in aqueous solutions under visible light illumination via a self-diffusiophoresis mechanism. Moreover, these micromachines can degrade toxic organic pollutants and respond to an increase in acidity of aqueous environments by instantaneous colour change. The combination of autonomous motility and intrinsic fluorescence enables these organic micromotors to be used as colorimetric and optical sensors for monitoring of the environmental aqueous acidity. The current findings open new pathways toward the design of organic polymer-based micromotors with tuneable band gap architecture for fabrication of self-propelled microsensors for environmental control and remediation applications.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

  • Continuities

    O - Projekt operacniho programu

Others

  • Publication year

    2020

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Advanced Functional Materials

  • ISSN

    1616-301X

  • e-ISSN

  • Volume of the periodical

    30

  • Issue of the periodical within the volume

    38

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    9

  • Pages from-to

  • UT code for WoS article

    000551442300001

  • EID of the result in the Scopus database

    2-s2.0-85088403840