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Ambient-temperature porogen-free method for preparation of silica-based macroporous materials

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F22%3A43925009" target="_blank" >RIV/60461373:22310/22:43925009 - isvavai.cz</a>

  • Alternative codes found

    RIV/60461373:22330/22:43925009 RIV/60461373:22340/22:43925009

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S0927775721019026?via%3Dihub" target="_blank" >https://www.sciencedirect.com/science/article/pii/S0927775721019026?via%3Dihub</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.colsurfa.2021.128033" target="_blank" >10.1016/j.colsurfa.2021.128033</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Ambient-temperature porogen-free method for preparation of silica-based macroporous materials

  • Original language description

    The presented work focuses on the synthesis of silica-based macroporous aggregates composed of silica nano-particles using a template-free method. To improve the mechanical strength of the prepared fractal-like aggregates, the silica precursor tetraethyl orthosilicate (TEOS) is used during nanoparticle aggregation. The obtained results confirm the possibility to tailor the pore size distribution (PSD) simply by using primary particles of various sizes. The prepared porous materials have a porosity ranging from 60% to 74% with a specific surface area between 10 and 200 m(2)/g and an average pore diameter from 30 to 1300 nm. Functionalization of the aggregate surface was done by replacing part of TEOS with a silica precursor that contained desired functional groups. This was demonstrated by preparing macroporous aggregates with carboxyl, amine and epoxy functional groups. The application of prepared aggregates was demonstrated by immobilization of urease from Canavalia ensiformis resulting in high enzyme activity compare to free enzymes.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20401 - Chemical engineering (plants, products)

Result continuities

  • Project

    <a href="/en/project/GA16-22997S" target="_blank" >GA16-22997S: Preparation of Porous Materials by Controlled Assembly of Nanoparticles</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2022

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Colloids and Surfaces A: Physicochemical and Engineering Aspects

  • ISSN

    0927-7757

  • e-ISSN

    1873-4359

  • Volume of the periodical

    634

  • Issue of the periodical within the volume

    FEB 5 2022

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    11

  • Pages from-to

    128033

  • UT code for WoS article

    000730865600005

  • EID of the result in the Scopus database

    2-s2.0-85120619979