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Hydrogen-Terminated Two-Dimensional Germanane/Silicane Alloys as Self-Powered Photodetectors and Sensors

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22310%2F23%3A43927542" target="_blank" >RIV/60461373:22310/23:43927542 - isvavai.cz</a>

  • Result on the web

    <a href="https://pubs.acs.org/doi/full/10.1021/acsami.3c01971" target="_blank" >https://pubs.acs.org/doi/full/10.1021/acsami.3c01971</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acsami.3c01971" target="_blank" >10.1021/acsami.3c01971</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Hydrogen-Terminated Two-Dimensional Germanane/Silicane Alloys as Self-Powered Photodetectors and Sensors

  • Original language description

    2D monoelementalmaterials, particularly germanene andsilicene(the single layer of germanium and silicon), which are the base materialsfor modern electronic devices demonstrated tremendous attraction fortheir 2D layer structure along with the tuneable electronics and opticalband gap. The major shortcoming of synthesized thermodynamically veryunstable layered germanene and silicene with their inclination towardoxidation was overcome by topochemical deintercalation of a Zintlphase (CaGe2, CaGe1.5Si0.5, and CaGeSi)in a protic environment. Theexfoliated Ge-H, Ge0.75Si0.25H, and Ge0.5Si0.5H were successfully synthesized and employedas the active layer for photoelectrochemical photodetectors, whichshowed broad response (420-940 nm), unprecedented responsivity,and detectivity on the order of 168 mu A W-1 and 3.45 x 10(8) cm Hz(1/2) W-1, respectively. The sensing capability of exfoliated germanane andsilicane composites was explored using electrochemical impedance spectroscopywith ultrafast response and recovery time of less than 1 s. Thesepositive findings serve as the application of exfoliated germaneneand silicene composites and can pave a new path to practical applicationsin efficient future devices.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10405 - Electrochemistry (dry cells, batteries, fuel cells, corrosion metals, electrolysis)

Result continuities

  • Project

    <a href="/en/project/GX19-26910X" target="_blank" >GX19-26910X: The chemistry in two dimensions - beyond graphene</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    ACS Applied Materials &amp; Interfaces

  • ISSN

    1944-8244

  • e-ISSN

    1944-8252

  • Volume of the periodical

    15

  • Issue of the periodical within the volume

    21

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    11

  • Pages from-to

    25693-25703

  • UT code for WoS article

    001014110200001

  • EID of the result in the Scopus database

    2-s2.0-85160678047