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Experimental and Computational Study on Liquid-Liquid Equilibrium in Ternary Systems of gamma-Valerolactone, Toluene, and Hydrocarbons

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22340%2F16%3A43900372" target="_blank" >RIV/60461373:22340/16:43900372 - isvavai.cz</a>

  • Result on the web

    <a href="http://pubs.acs.org/doi/abs/10.1021/acs.jced.5b00611" target="_blank" >http://pubs.acs.org/doi/abs/10.1021/acs.jced.5b00611</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1021/acs.jced.5b00611" target="_blank" >10.1021/acs.jced.5b00611</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Experimental and Computational Study on Liquid-Liquid Equilibrium in Ternary Systems of gamma-Valerolactone, Toluene, and Hydrocarbons

  • Original language description

    ?-Valerolactone is a biomass-derived compound widely applicable in chemical industry, especially as a solvent, additive to fuels or precursor for other chemicals. In contrast with the industrial importance of ?-valerolactone, there is an insufficient number of mixture phase-equilibria in the literature. Therefore the aim of this work was to measure liquid-liquid equilibrium data for ternary systems ?-valerolactone + toluene + hydrocarbon (hydrocarbons were n-heptane, n-decane, n-dodecane, and cyclohexane) by the direct analytical method at 298.15 K and 0.1 MPa. The obtained experimental data were processed and correlated by the nonrandom two-liquid (NRTL) model. The NRTL binary parameters between ?-valerolactone and toluene were evaluated from the measured ternary liquid-liquid equilibrium data while the other binary parameters were obtained by regression of binary liquid-liquid equilibrium data or vapor-liquid equilibrium and excess enthalpy data taken from literature. The predictive performance of the perturbed-chain induced-polar SAFT (PCIP-SAFT) equation of state was also studied for the ternary systems. Based on the pure-components data only, the PCIP-SAFT predictions can be considered as relatively successful because of the ability of PCIP-SAFT to take into account the dipolar interactions.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2016

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Chemical Engineering Data

  • ISSN

    0021-9568

  • e-ISSN

  • Volume of the periodical

    61

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    7

  • Pages from-to

    391-397

  • UT code for WoS article

    000368564600044

  • EID of the result in the Scopus database