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Pickup and Photodissociation of Hydrogen Halides in Floppy Neon Clusters.

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F03%3A54030144" target="_blank" >RIV/61388955:_____/03:54030144 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Pickup and Photodissociation of Hydrogen Halides in Floppy Neon Clusters.

  • Original language description

    Neon clusters with an average sizes in the range from n=100 to 1600 atoms are generated in an adiabatic expansion and are doped with a single HBr or HCl molecule in a pick-up process. The hydrogen halide molecule is photodissociated by a UV laser and theoutgoing H fragment is ionized by resonance enhanced multi-photon ionization (REMPI) in a (2+1) excitation scheme at a wavelength of 243 nm. The H ions are extracted in a Wiley-McLaren time-of-flight mass spectrometer operating in the low-field mode tobe sensitive to low velocities. Themeasured kinetic energy distribution are compared with quasi-classical molecular dynamics simulations, which allow for a detailed analysis of the underlying processes. Simultaneously, the neon cluster phase behavior, the pick-up procedure, and the photodissociation dynamics are investigated theoretically. The phase behavior is studied by means of the Instantaneous Normal Modes approach with a newly introduced projection technique.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/LN00A032" target="_blank" >LN00A032: Structure and dynamics of complex molecular systems and biomolecules</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2003

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Physical Chemistry. A

  • ISSN

    1089-5639

  • e-ISSN

  • Volume of the periodical

    107

  • Issue of the periodical within the volume

    N/A

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    12

  • Pages from-to

    7743-7754

  • UT code for WoS article

  • EID of the result in the Scopus database