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High activity of iron containing metal-organic-framework in acylation of p-xylene with benzoyl chloride

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F12%3A00375913" target="_blank" >RIV/61388955:_____/12:00375913 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1016/j.cattod.2011.08.001" target="_blank" >http://dx.doi.org/10.1016/j.cattod.2011.08.001</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.cattod.2011.08.001" target="_blank" >10.1016/j.cattod.2011.08.001</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    High activity of iron containing metal-organic-framework in acylation of p-xylene with benzoyl chloride

  • Original language description

    Catalytic behavior of metal-organic-frameworks (MOFs) Cu-3(BTC)(2), MIL-100(Fe) and MIL-100(Cr) was investigated in p-xylene acylation with benzoyl chloride and compared with the behavior of large pore zeolites Beta and USY. It has been clearly shown that MIL-100(Fe) exhibit much higher conversion of benzoyl chloride with excellent selectivity in p-xylene acylation. The performance of MIL-100(Fe) catalyst was favorable with those of other conventional heterogeneous catalysts like zeolites. Conversion ofbenzoyl chloride equal to 100% was achieved over MIL-100(Fe) with 20-30 min under optimized reaction conditions. It is assumed that unsaturated Lewis acid sites associated with the presence of Fe exhibit optimum acid strength for catalyzing this acylation reaction.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA104%2F07%2F0383" target="_blank" >GA104/07/0383: Development of new heterogeneous catalysts for acylation reactions</a><br>

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2012

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Catalysis Today

  • ISSN

    0920-5861

  • e-ISSN

  • Volume of the periodical

    179

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    6

  • Pages from-to

    85-90

  • UT code for WoS article

    000298404600011

  • EID of the result in the Scopus database