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Tracking all-vapor instant gas-hydrate formation and guest molecule populations: A possible probe for molecules trapped in water nanodroplets

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F12%3A00384412" target="_blank" >RIV/61388955:_____/12:00384412 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1063/1.4767370" target="_blank" >http://dx.doi.org/10.1063/1.4767370</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1063/1.4767370" target="_blank" >10.1063/1.4767370</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Tracking all-vapor instant gas-hydrate formation and guest molecule populations: A possible probe for molecules trapped in water nanodroplets

  • Original language description

    Quantitative Fourier-transform infrared spectra for low-temperature (160?200 K) aerosols of clathrate-hydrate nanoparticles that contain large-cage catalysts and small-cage nonpolar guests have been extended to a broad range of vapor compositions and sampling conditions. The data better reveal the stages by which room-temperature vapor mixtures, when cooled below 220 K, instantly generate aerosols with particles composed exclusively of the corresponding clathrate hydrates. In particular the quantitativedata help relate the nature of the hydrates that form to the composition of the aqueous nanodroplets of the first stages of the rapid transition from the all-vapor mixture. The overall transition from an all-vapor mixture to ?gas-hydrate nanocrystals isa multistage one that has been characterized as homogeneous nucleation and growth of solution nanodroplets (240 K) followed by nucleation and growth of the gas-hydrate particles (220 K); all occurring within a subsecond that follows puls

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2012

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Chemical Physics

  • ISSN

    0021-9606

  • e-ISSN

  • Volume of the periodical

    137

  • Issue of the periodical within the volume

    20

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    12

  • Pages from-to

  • UT code for WoS article

    000312252100042

  • EID of the result in the Scopus database