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Energy and charge transfer in ionized argon coated water clusters

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F13%3A00420663" target="_blank" >RIV/61388955:_____/13:00420663 - isvavai.cz</a>

  • Alternative codes found

    RIV/60461373:22340/13:43895772

  • Result on the web

    <a href="http://dx.doi.org/10.1063/1.4834715" target="_blank" >http://dx.doi.org/10.1063/1.4834715</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1063/1.4834715" target="_blank" >10.1063/1.4834715</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Energy and charge transfer in ionized argon coated water clusters

  • Original language description

    We investigate the electron ionization of clusters generated in mixed Ar-water expansions. The electron energy dependent ion yields reveal the neutral cluster composition and structure: water clusters fully covered with the Ar solvation shell are formedunder certain expansion conditions. The argon atoms shield the embedded (H 2 O) n clusters resulting in the ionization threshold above 15 eV for all fragments. The argon atoms also mediate more complex reactions in the clusters: e.g., the charge transferbetween Ar + and water occurs above the threshold; at higher electron energies above 28 eV, an excitonic transfer process between Ar + * and water opens leading to new products Ar n H + and (H 2 O) n H + . On the other hand, the excitonic transfer fromthe neutral Ar* state at lower energies is not observed although this resonant process was demonstrated previously in a photoion- ization experiment. Doubly charged fragments (H 2 O) n H 2 + 2 and (H 2 O) 2 + n ions are observed and In- t

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GAP208%2F11%2F0161" target="_blank" >GAP208/11/0161: Dynamicss of Solvated Electrons in Molecular Clusters: Experimental and Theoretical Approach</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2013

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Chemical Physics

  • ISSN

    0021-9606

  • e-ISSN

  • Volume of the periodical

    139

  • Issue of the periodical within the volume

    21

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    7

  • Pages from-to

  • UT code for WoS article

    000328636400026

  • EID of the result in the Scopus database