Energy and charge transfer in ionized argon coated water clusters

Result code in IS VaVaI
<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F13%3A00420663" target="_blank" >RIV/61388955:_____/13:00420663 - isvavai.cz</a>
Alternative codes found
RIV/60461373:22340/13:43895772
Result on the web
<a href="http://dx.doi.org/10.1063/1.4834715" target="_blank" >http://dx.doi.org/10.1063/1.4834715</a>
DOI - Digital Object Identifier
<a href="http://dx.doi.org/10.1063/1.4834715" target="_blank" >10.1063/1.4834715</a>

Result language
angličtina
Original language name
Energy and charge transfer in ionized argon coated water clusters
Original language description
We investigate the electron ionization of clusters generated in mixed Ar-water expansions. The electron energy dependent ion yields reveal the neutral cluster composition and structure: water clusters fully covered with the Ar solvation shell are formedunder certain expansion conditions. The argon atoms shield the embedded (H 2 O) n clusters resulting in the ionization threshold above 15 eV for all fragments. The argon atoms also mediate more complex reactions in the clusters: e.g., the charge transferbetween Ar + and water occurs above the threshold; at higher electron energies above 28 eV, an excitonic transfer process between Ar + * and water opens leading to new products Ar n H + and (H 2 O) n H + . On the other hand, the excitonic transfer fromthe neutral Ar* state at lower energies is not observed although this resonant process was demonstrated previously in a photoion- ization experiment. Doubly charged fragments (H 2 O) n H 2 + 2 and (H 2 O) 2 + n ions are observed and In- t
Czech name
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Czech description
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Type
J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)
CEP classification
CF - Physical chemistry and theoretical chemistry
OECD FORD branch
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Project
<a href="/en/project/GAP208%2F11%2F0161" target="_blank" >GAP208/11/0161: Dynamicss of Solvated Electrons in Molecular Clusters: Experimental and Theoretical Approach</a><br>
Continuities
I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Publication year
2013
Confidentiality
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

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