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Measurement of line strengths in the à <sup>2</sup>A’ ← X˜ <sup>2</sup>A” transition of HO<inf>2</inf> and DO<inf>2</inf>

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F17%3A00506626" target="_blank" >RIV/61388955:_____/17:00506626 - isvavai.cz</a>

  • Result on the web

    <a href="http://hdl.handle.net/11104/0297835" target="_blank" >http://hdl.handle.net/11104/0297835</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.jqsrt.2017.07.004" target="_blank" >10.1016/j.jqsrt.2017.07.004</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Measurement of line strengths in the à <sup>2</sup>A’ ← X˜ <sup>2</sup>A” transition of HO<inf>2</inf> and DO<inf>2</inf>

  • Original language description

    The absorption spectrum of the à 2A’ ← X˜ 2A” 000–000 band of HO2 and DO2 radicals has been measured in the range 6941–7077 cm−1 with a resolution of around 0.005 cm−1. HO2 and DO2 radicals were generated from the reaction of Cl-atoms with CH3OH and CD3OD, respectively, whereby Cl-atoms were generated by pulsed photolysis of (COCl)2 at 248 nm. One time-resolved absorption curve was measured by cw-Cavity Ring Down Spectroscopy (cw-CRDS) for each wavelength. The relative absorption coefficient for each wavelength was then obtained from the ring down time τ, extrapolated to t = 0 s with respect to the photolysis pulse, and the ring down time τ0 before the photolysis pulse. Absolute absorption coefficients were quantified for several selected lines relative to a well characterized absorption line of HO2 at 6638.21 cm−1 by a second cw-CRDS absorption path. The maximum absorption cross section at 50 Torr Helium was for HO2 the transition N Ka Kc J = 11 0 11 11.5 ← 11 1 11 11.5 with σ7000.28 cm−1 = 2.12 × 10−19 cm2 and for DO2 the doublet transition N Ka Kc J = 18 1 18 18.5 ← 18 0 18 18.5 and 18 1 18 17.5 ← 18 0 18 17.5 with σ7019.83 cm−1 = 2.97 × 10−19 cm2. The full spectrum has been very well reproduced by employing spectroscopic data from earlier works.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2017

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Quantitative Spectroscopy and Radiative Transfer

  • ISSN

    0022-4073

  • e-ISSN

  • Volume of the periodical

    201

  • Issue of the periodical within the volume

    NOV 2017

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    10

  • Pages from-to

    161-170

  • UT code for WoS article

    000411544100017

  • EID of the result in the Scopus database

    2-s2.0-85024131324