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Dissociative electron attachment to HNO3 and its hydrates: energy-selective electron-induced chemistry

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F19%3A00504200" target="_blank" >RIV/61388955:_____/19:00504200 - isvavai.cz</a>

  • Result on the web

    <a href="http://hdl.handle.net/11104/0295880" target="_blank" >http://hdl.handle.net/11104/0295880</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1039/C9CP00990F" target="_blank" >10.1039/C9CP00990F</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Dissociative electron attachment to HNO3 and its hydrates: energy-selective electron-induced chemistry

  • Original language description

    We probe the negative ion production upon the interaction of free electrons with gas-phase HNO3 and its mixed clusters with water. The electron-induced chemistry changes strongly with clustering, exhibiting significant electron energy dependence. For HNO3 hydrates, we identified three involved energy ranges with different behavior: low energies up to about 3.5 eV, an intermediate energy range around 6 eV, and a high energy range, approximately above 9 eV. The major difference is the degree to which the major gas-phase product, NO2−, is converted to NO3−. The latter is the dominant stratospheric anion. Its appearance due to the electron interaction with mixed HNO3/water ice particles thus strongly depends on the electron energy. We discuss the elementary processes and reaction pathways behind the anion conversion.n

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Physical Chemistry Chemical Physics

  • ISSN

    1463-9076

  • e-ISSN

  • Volume of the periodical

    21

  • Issue of the periodical within the volume

    APR 2019

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    7

  • Pages from-to

    8691-8697

  • UT code for WoS article

    000474599300005

  • EID of the result in the Scopus database

    2-s2.0-85065174694