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Cobalt pyridinoporphyrazine film as a platinum group metal-free mediator in hydrogen electrochemistry

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F19%3A00508539" target="_blank" >RIV/61388955:_____/19:00508539 - isvavai.cz</a>

  • Alternative codes found

    RIV/00216208:11310/19:10399166

  • Result on the web

    <a href="http://hdl.handle.net/11104/0299411" target="_blank" >http://hdl.handle.net/11104/0299411</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s00706-019-02452-0" target="_blank" >10.1007/s00706-019-02452-0</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Cobalt pyridinoporphyrazine film as a platinum group metal-free mediator in hydrogen electrochemistry

  • Original language description

    The cobalt pyridinoporphyrazine film deposited on basal plane highly oriented pyrolytic graphite (HOPG) and Au(111) electrodes exhibited electrocatalytic activity to hydrogen oxidation reaction compared to the bare electrode surfaces. The deposition performed by spontaneous adsorption of the cobalt pyridinoporphyrazine complex from its aqueous solution led on basal plane HOPG to the formation of a uniform homogeneous film with simultaneous reduction of cobalt centre, while at Au(111) electrode preferential aggregation of pyridinoporphyrazine complex took place without any change of reduction state of cobalt. Accordingly, both substrates affected the pathway of electrocatalytic hydrogen oxidation. Potentiometric detection of hydrogen based on equilibrium potential of pyridinoporphyrazine Co(II)/Co(I) electrode upon alternation presence of hydrogen and argon in solution was examined.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10405 - Electrochemistry (dry cells, batteries, fuel cells, corrosion metals, electrolysis)

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2019

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Monatshefte fur Chemie

  • ISSN

    0026-9247

  • e-ISSN

  • Volume of the periodical

    150

  • Issue of the periodical within the volume

    9

  • Country of publishing house

    AT - AUSTRIA

  • Number of pages

    8

  • Pages from-to

    1643-1650

  • UT code for WoS article

    000482907600013

  • EID of the result in the Scopus database

    2-s2.0-85070187530