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Synthesis and computational mechanistic studies of copper selective molecular receptor

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F20%3A00538019" target="_blank" >RIV/61388955:_____/20:00538019 - isvavai.cz</a>

  • Result on the web

    <a href="http://hdl.handle.net/11104/0315850" target="_blank" >http://hdl.handle.net/11104/0315850</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/vjch.201900161" target="_blank" >10.1002/vjch.201900161</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Synthesis and computational mechanistic studies of copper selective molecular receptor

  • Original language description

    Although numerous molecular receptors for Cu2+ have been reported, it is not obvious to find a simple molecule as a selective receptor for Cu2+. Here we create a molecular receptor 4MHEB for Cu2+ metal ions. Observation of a new absorption band near 282 nm in UV-visible spectra and enhancement in fluorescence intensity in emission spectra justify the binding 4MHEB:Cu2+ binding. Inspection in shifting of IR bands, different thermal behavior and oxidation and reduction peaks of complex shows binding of 4MHEB:Cu2+. HRMS m/z 322.0328, Benesi-Hildebrand method and Job's Plot results 1:1 (4MHEB:Cu2+) binding stoichiometry with the binding affinity K = 1.751x10(5) M-1. The docked pose of 4MHEB with Cu2+ ion, Key transitions, % Contribution was calculated by computational studies.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

    <a href="/en/project/GA17-18108S" target="_blank" >GA17-18108S: Novel electrochemically active thiacalix[4]arenes and their oxidized analogues as ligands and receptors</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2020

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    VIETNAM JOURNAL OF CHEMISTRY

  • ISSN

    0866-7144

  • e-ISSN

  • Volume of the periodical

    58

  • Issue of the periodical within the volume

    2

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    10

  • Pages from-to

    221-230

  • UT code for WoS article

    000588009800014

  • EID of the result in the Scopus database